A global assessment of precipitation chemistry and deposition has been carried out under the direction of the World Meteorological Organization (WMO) Global Atmosphere Watch (GAW) Scientific Advisory ...Group for Precipitation Chemistry (SAG-PC). The assessment addressed three questions: (1) what do measurements and model estimates of precipitation chemistry and wet, dry and total deposition of sulfur, nitrogen, sea salt, base cations, organic acids, acidity, and phosphorus show globally and regionally? (2) has the wet deposition of major ions changed since 2000 (and, where information and data are available, since 1990) and (3) what are the major gaps and uncertainties in our knowledge? To that end, regionally-representative measurements for two 3-year-averaging periods, 2000–2002 and 2005–2007, were compiled worldwide. Data from the 2000–2002 averaging period were combined with 2001 ensemble-mean modeling results from 21 global chemical transport models produced in Phase 1 of the Coordinated Model Studies Activities of the Task Force on Hemispheric Transport of Air Pollution (TF HTAP). The measurement data and modeling results were used to generate global and regional maps of major ion concentrations in precipitation and deposition. A major product of the assessment is a database of quality assured ion concentration and wet deposition data gathered from regional and national monitoring networks. The database is available for download from the World Data Centre for Precipitation Chemistry (http://wdcpc.org/). The assessment concludes that global concentrations and deposition of sulfur and nitrogen are reasonably well characterized with levels generally highest near emission sources and more than an order of magnitude lower in areas largely free of anthropogenic influences. In many parts of the world, wet deposition of reduced nitrogen exceeds that of oxidized nitrogen and is increasing. Sulfur and nitrogen concentrations and deposition in North America and Europe have declined significantly in line with emission reduction policies. Major regions of the world, including South America, the more remote areas of North America, much of Asia, Africa, Oceania, polar regions, and all of the oceans, are inadequately sampled for all of the major ions in wet and dry deposition, and particularly so for phosphorus, organic forms of nitrogen, and weak acids including carbonates and organic acids. Measurement-based inferential estimates of dry deposition are limited to sulfur and some nitrogen in only a few regions of the world and methods are highly uncertain. The assessment concludes with recommendations to address major gaps and uncertainties in global ion concentration and deposition measurements.
•Assessed the global distribution of precipitation composition and deposition of major ions.•Produced a global data set of quality assured wet deposition monitoring data for 2000–2002 and 2005–2007.•Generated global wet deposition maps of major ions combining measurement and modeling results.•Established that sulfur and nitrogen wet deposition is highest in parts of Asia, Europe and eastern North America.•Determined that major gaps in wet and dry deposition monitoring exist globally.
Ice particles in high-altitude cold clouds can obstruct aircraft functioning. Over the last 20 years, there have been more than 150 recorded cases with engine power-loss and damage caused by tiny ...cloud ice crystals, which are difficult to detect with aircraft radars. Herein, we examine two aircraft accidents for which icing linked to convective weather conditions has been officially reported as the most likely reason for catastrophic consequences. We analyze whether desert mineral dust, known to be very efficient ice nuclei and present along both aircraft routes, could further augment the icing process. Using numerical simulations performed by a coupled atmosphere-dust model with an included parameterization for ice nucleation triggered by dust aerosols, we show that the predicted ice particle number sharply increases at approximate locations and times of accidents where desert dust was brought by convective circulation to the upper troposphere. We propose a new icing parameter which, unlike existing icing indices, for the first time includes in its calculation the predicted dust concentration. This study opens up the opportunity to use integrated atmospheric-dust forecasts as warnings for ice formation enhanced by mineral dust presence.
This paper reviews our knowledge of the measurement and modeling of mineral dust emissions to the atmosphere, its transport and deposition to the ocean, the release of iron from the dust into ...seawater, and the possible impact of that nutrient on marine biogeochemistry and climate. Of particular concern is our poor understanding of the mechanisms and quantities of dust deposition as well as the extent of iron solubilization from the dust once it enters the ocean. Model estimates of dust deposition in remote oceanic regions vary by more than a factor of 10. The fraction of the iron in dust that is available for use by marine phytoplankton is still highly uncertain. There is an urgent need for a long-term marine atmospheric surface measurement network, spread across all oceans. Because the southern ocean is characterized by large areas with high nitrate but low chlorophyll surface concentrations, that region is particularly sensitive to the input of dust and iron. Data from this region would be valuable, particularly at sites downwind from known dust source areas in South America, Australia, and South Africa. Coordinated field experiments involving both atmospheric and marine measurements are recommended to address the complex and interlinked processes and role of dust/Fe fertilization on marine biogeochemistry and climate.
Inclusion of mineral dust radiative effects could lead to a significant improvement in the radiation balance of numerical weather prediction models with subsequent improvements in the weather ...forecast itself. In this study the radiative effects of mineral dust have been fully incorporated into a regional atmospheric dust model. Dust affects the radiative fluxes at the surface and the top of the atmosphere and the temperature profiles at every model time step when the radiation module is processed. These changes influence the atmospheric dynamics, moisture physics, and near‐surface conditions. Furthermore, dust emission is modified by changes in friction velocity and turbulent exchange coefficients; dust turbulent mixing, transport, and deposition are altered by changes in atmospheric stability, precipitation conditions, and free‐atmosphere winds. A major dust outbreak with dust optical depths reaching 3.5 at 550 nm over the Mediterranean region on April 2002 is selected to assess the radiative dust effects on the atmosphere at a regional level. A strong dust negative feedback upon dust emission (35–45% reduction of the AOD) resulted from the smaller outgoing sensible turbulent heat flux decreasing the turbulent momentum transfer from the atmosphere and consequently dust emission. Significant improvements of the atmospheric temperature and mean sea‐level pressure forecasts are obtained over dust‐affected areas by considerably reducing both warm and cold temperature biases existing in the model without dust‐radiation interactions. This study demonstrates that the use of the proposed model with integrated dust and atmospheric radiation represents a promising approach for further improvements in numerical weather prediction practice and radiative impact assessment over dust‐affected areas.
Long‐range transport of desert dust from the Sahara across the northern Atlantic has been recorded many times by satellite imagery and ground‐based measurements. However, this evidence cannot fully ...describe all the phases of the atmospheric dust lifecycle. To partly compensate for the lack of such knowledge, an atmospheric model with incorporated dust uptake‐transport‐deposition module has been used in this study. The goal was to assess qualitatively and quantitatively the ability of the model to predict the dust cycle in the atmosphere for a long period. For this purpose, the complicated dust episode of June–July 1993 (almost one month) was simulated with the SKIRON weather forecasting system. This dust intrusion was associated with long‐range transport of Saharan dust across the Atlantic Ocean and simultaneous regional transport towards the Mediterranean Sea. Comparison of the forecasts with the available observations (in a qualitative and quantitatively way) indicated that the model was able to simulate the long‐range dust transport patterns and in particular to estimate the spatiotemporal distribution of the dust concentration on a satisfactory way.
An integrated modeling system has been developed to accurately describe the dust cycle in the atmosphere. It is based on the SKIRON/Eta modeling system and the Eta/NCEP regional atmospheric model. ...The dust modules of the entire system incorporate the state of the art parameterizations of all the major phases of the atmospheric dust life such as production, diffusion, advection, and removal. These modules also include effects of the particle size distribution on aerosol dispersion. The dust production mechanism is based on the viscous/turbulent mixing, shear‐free convection diffusion, and soil moisture. In addition to these sophisticated mechanisms, very high resolution databases, including elevation, soil properties, and vegetation cover are utilized. The entire system is easily configurable and transferable to any place on the Earth, it can cover domains on almost any size, and its horizontal resolution can vary from about 100 km up to approximately 4 km. It can run on one‐way‐nested form if necessary. The performance of the system has been tested for various dust storm episodes, in various places and resolution using gridded analysis or forecasting fields from various sources (ECMWF and NCEP) for initial and boundary conditions. The system is in operational use during the last two years, providing 72 hour forecasts for the Mediterranean region. The results are available on the internet (http://www.icod.org.mt and http://forecast.uoa.gr).
Dust Dry Deposition over Israel Kishcha, Pavel; Volpov, Evgeni; Starobinets, Boris ...
Atmosphere,
02/2020, Letnik:
11, Številka:
2
Journal Article
Recenzirano
Odprti dostop
Similar quasiperiodic year-to-year variations of dust dry deposition (DDD) with a two–three-year period were found over Israel and north-east Africa. This phenomenon of quasiperiodic interannual ...variations of DDD has not been discussed in previous publications. Moreover, similar seasonal variations of DDD were found over both Israel and north-east Africa, characterized by significant dust deposition in spring and a decrease in DDD from spring to autumn. These findings indicate the existence of the same causal factors for interannual and seasonal variations of DDD over the two regions, such as similar surface winds created by Mediterranean cyclones. Daily runs of the Dust REgional Atmospheric Model (DREAM) at Tel Aviv University from 2006 to 2019 were used to investigate the main features of the spatio-temporal distribution of dust dry deposition in the eastern Mediterranean, with a focus on Israel. DREAM showed that, on average, during the 14-year study period, in the winter, spring, and summer months, the spatial distribution of monthly-accumulated DDD over Israel was non-uniform with the maximum of DDD over southern Israel. In the autumn months, DREAM showed an increase in DDD over northern Israel, resulting in an almost uniform DDD pattern. The knowledge of DDD spatio-temporal distribution is helpful for understanding the negative effects of DDD on the performance of solar panels and on insulator flashover in the Israel power electric network.
We present the development of a physically-based dust source map for the GOCART-AFWA dust module in WRF-Chem model. The new parameterization is based on MODIS-NDVI and an updated emission strength ...map is computed every 15 days from the latest satellite observations. Modeling simulations for the period April–May 2017 over the Mediterranean, north Africa, and the Middle East are compared with observations of AOD at 31 AERONET stations. The new module is capable of reproducing the dust sources at finer detail. The overall performance of the model is improved, especially for stronger dust episodes with AOD > 0.25. For this threshold the model BIAS decreases from −0.20 to −0.02, the RMSE from 0.38 to 0.30, the Correlation Coefficient improves from 0.21 to 0.47, the fractional gross error (FGE) from 0.62 to 0.40, and the mean fractional bias (MFB) from −0.49 to −0.08. Similar improvement is also found for the lower AOD thresholds (>0.0 and >0.1), especially for the stations in Europe, the Mediterranean, Sahel, the Middle East, and Arabian Peninsula, which are mostly affected by dust transport during the experimental period. An overprediction of AOD, compared to the original dust-source scheme, is found for some stations in the Sahara desert, the Atlantic Ocean, and the Iberian Peninsula. In total, 124 out of the 170 statistical scores that are calculated indicate improvement of model performance.
The mineralogical composition of airborne dust particles is an important but often neglected parameter for several physiochemical processes, such as atmospheric radiative transfer and ocean ...biochemistry. We present the development of the METAL-WRF module for the simulation of the composition of desert dust minerals in atmospheric aerosols. The new development is based on the GOCART-AFWA dust module of WRF-Chem. A new wet deposition scheme has been implemented in the dust module alongside the existing dry deposition scheme. The new model includes separate prognostic fields for nine (9) minerals: illite, kaolinite, smectite, calcite, quartz, feldspar, hematite, gypsum, and phosphorus, derived from the GMINER30 database and also iron derived from the FERRUM30 database. Two regional model sensitivity studies are presented for dust events that occurred in August and December 2017, which include a comparison of the model versus elemental dust composition measurements performed in the North Atlantic (at Izaña Observatory, Tenerife Island) and in the eastern Mediterranean (at Agia Marina Xyliatos station, Cyprus Island). The results indicate the important role of dust minerals, as dominant aerosols, for the greater region of North Africa, South Europe, the North Atlantic, and the Middle East, including the dry and wet depositions away from desert sources. Overall, METAL-WRF was found to be capable of reproducing the relative abundances of the different dust minerals in the atmosphere. In particular, the concentration of iron (Fe), which is an important element for ocean biochemistry and solar absorption, was modeled in good agreement with the corresponding measurements at Izaña Observatory (22% overestimation) and at Agia Marina Xyliatos site (4% overestimation). Further model developments, including the implementation of newer surface mineralogical datasets, e.g., from the NASA-EMIT satellite mission, can be implemented in the model to improve its accuracy.
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