The ability to confine light into tiny spatial dimensions is important for applications such as microscopy, sensing, and nanoscale lasers. Although plasmons offer an appealing avenue to confine ...light, Landau damping in metals imposes a trade-off between optical field confinement and losses. We show that a graphene-insulator-metal heterostructure can overcome that trade-off, and demonstrate plasmon confinement down to the ultimate limit of the length scale of one atom. This is achieved through far-field excitation of plasmon modes squeezed into an atomically thin hexagonal boron nitride dielectric spacer between graphene and metal rods. A theoretical model that takes into account the nonlocal optical response of both graphene and metal is used to describe the results. These ultraconfined plasmonic modes, addressed with far-field light excitation, enable a route to new regimes of ultrastrong light-matter interactions.
The extreme electro-optical contrast between crystalline and amorphous states in phase-change materials is routinely exploited in optical data storage and future applications include universal ...memories, flexible displays, reconfigurable optical circuits, and logic devices. Optical contrast is believed to arise owing to a change in crystallinity. Here we show that the connection between optical properties and structure can be broken. Using a combination of single-shot femtosecond electron diffraction and optical spectroscopy, we simultaneously follow the lattice dynamics and dielectric function in the phase-change material Ge2Sb2Te5 during an irreversible state transformation. The dielectric function changes by 30% within 100 fs owing to a rapid depletion of electrons from resonantly bonded states. This occurs without perturbing the crystallinity of the lattice, which heats with a 2-ps time constant. The optical changes are an order of magnitude larger than those achievable with silicon and present new routes to manipulate light on an ultrafast timescale without structural changes.
A compact pin Ge photodetector is integrated in submicron SOI rib waveguide. The detector length is reduced down to 15 microm using butt coupling configuration which is sufficient to totally absorb ...light at the wavelength of 1.55 microm. A -3 dB bandwidth of 42 GHz has been measured at a 4V reverse bias with a responsivity as high as 1 A/W at the wavelength of 1.55 microm and a low dark current density of 60 mA/cm(2). At a wavelength of 1.52 microm, a responsivity of 1 A/W is obtained under -0.5 V bias. The process is fully compatible with CMOS technology.
Polarization control through all-dielectric metasurfaces holds great potential in different fields, such as telecommunications, biochemistry and holography. Asymmetric chiral metasurfaces supporting ...quasi-bound states in the continuum may prove very useful for controlling and manipulating the polarization state of light. A crucial quantity for characterizing the optical chirality is the circular dichroism (CD). In this work we analyse how the CD and quality factor of the optical mode can be strongly influenced by a nanofabrication error. Modelling the nanofabrication uncertainties on the gaps of the chiral metasurface, the imperfections of the etchings process or the modification of the asymmetry factor, we found that the proper engineering of the gap between the nanostructures of the unit cell is the most important parameter to achieve a high-quality factor and enhanced optical dichroism. An optimization of the nanofabrication processes, such as dose factor, dwell time and plasma etching demonstrates that, for a writing field of 100 μm2, it is possible to obtain morphologically precise chiral metasurfaces, with fabrication uncertainties lower than those that would limit Q factor and chirality property.
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•Engineering of an asymmetric Si metasurface to support Bound States in the Continuum (BICs) and optical chirality.•Numerical simulation of nanofabrication error influences on Third Harmonic Circular Dichroism and Q-Factor of the modes.•Detailed fabrication process of the metasurface on a 100 um2 write field with a 30 KV EBL.
One of the main limitations for achieving truly lab-on-a-chip (LOC) devices for point-of-care diagnosis is the incorporation of the "on-chip" detection. Indeed, most of the state-of-the-art LOC ...devices usually require complex read-out instrumentation, losing the main advantages of portability and simplicity. In this context, we present our last advances towards the achievement of a portable and label-free LOC platform with highly sensitive "on-chip" detection by using nanophotonic biosensors. Bimodal waveguide interferometers fabricated by standard silicon processes have been integrated with sub-micronic grating couplers for efficient light in-coupling, showing a phase resolution of 6.6 × 10(-4)× 2π rad and a limit of detection of 3.3 × 10(-7) refractive index unit (RIU) in bulk. A 3D network of SU-8 polymer microfluidics monolithically assembled at the wafer-level was included, ensuring perfect sealing and compact packaging. To overcome some of the drawbacks inherent to interferometric read-outs, a novel all-optical wavelength modulation system has been implemented, providing a linear response and a direct read-out of the phase variation. Sensitivity, specificity and reproducibility of the wavelength modulated BiMW sensor has been demonstrated through the label-free immunodetection of the human hormone hTSH at picomolar level using a reliable biofunctionalization process.
Fluorescence microscopy is the method of choice in biology for its molecular specificity and super-resolution capabilities. However, it is limited to a narrow
range around one observation plane. ...Here, we report an imaging approach that recovers the full electric field of fluorescent light with single-molecule sensitivity. We expand the principle of digital holography to fast fluorescent detection by eliminating the need for phase cycling and enable three-dimensional (3D) tracking of individual nanoparticles with an in-plane resolution of 15 nm and a
-range of 8 mm. As a proof-of-concept biological application, we image the 3D motion of extracellular vesicles (EVs) inside live cells. At short time scales (<4 s), we resolve near-isotropic 3D diffusion and directional transport. For longer lag times, we observe a transition toward anisotropic motion with the EVs being transported over long distances in the axial plane while being confined in the horizontal dimension.
Ultrafast transient microscopy is a key tool to study the photophysical properties of materials in space and time, but current implementations are limited to ≈1-μm fields of view, offering no ...statistical information for heterogeneous samples. Recently, we demonstrated wide-field transient imaging based on multiplexed off-axis holography. Here, we perform ultrafast microscopy in parallel around a hundred diffraction-limited excitation spots over a ≈60-μm field of view, which not only automatically samples the photophysical heterogeneity of the sample over a large area but can also be used to obtain a 10-fold increase in signal-to-noise ratio by computing an average spot. We apply our microscope to study the carrier diffusion processes in methylammonium lead bromide perovskites. We observe strong diffusion due to the presence of hot carriers during the first picosecond and slower diffusion afterward. We also describe how many-body kinetics can be misleadingly interpreted as strong diffusion at high excitation densities, while at weak excitation, real diffusion is observed. Therefore, the vast increase in sensitivity offered by this technique benefits the study of carrier transport not only by reducing data acquisition times but also by enabling the measurement of the much smaller signals generated at low carrier densities.
We present the design, fabrication, and characterization of submicronic grating couplers integrated on Si 3 N 4 rib waveguide Mach-Zehnder interferometers (MZIs) for biosensing applications working ...in the visible spectral range for both TE and TM polarizations. Depending on the waveguide structure, a maximum of 11.5% of coupling efficiency has been experimentally obtained at 658 nm, while a limit of detection of 1.6 × 10 -7 in refractive index unit is achieved for the biosensor. These results represent an important milestone toward the achievement of a truly portable and multiplexed point-of-care platform using the integrated MZI sensor.
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