Many advanced applications of X-ray free-electron lasers require pulse durations and time resolutions of only a few femtoseconds. To generate these pulses and to apply them in time-resolved ...experiments, synchronization techniques that can simultaneously lock all independent components, including all accelerator modules and all external optical lasers, to better than the delivered free-electron laser pulse duration, are needed. Here we achieve all-optical synchronization at the soft X-ray free-electron laser FLASH and demonstrate facility-wide timing to better than 30 fs r.m.s. for 90 fs X-ray photon pulses. Crucially, our analysis indicates that the performance of this optical synchronization is limited primarily by the free-electron laser pulse duration, and should naturally scale to the sub-10 femtosecond level with shorter X-ray pulses.
The ability to fully characterize ultrashort, ultra-intense X-ray pulses at free-electron lasers (FELs) will be crucial in experiments ranging from single-molecule imaging to extreme-timescale X-ray ...science. This issue is especially important at current-generation FELs, which are primarily based on self-amplified spontaneous emission and radiate with parameters that fluctuate strongly from pulse to pulse. Using single-cycle terahertz pulses from an optical laser, we have extended the streaking techniques of attosecond metrology to measure the temporal profile of individual FEL pulses with 5 fs full-width at half-maximum accuracy, as well as their arrival on a time base synchronized to the external laser to within 6 fs r.m.s. Optical laser-driven terahertz streaking can be utilized at any X-ray photon energy and is non-invasive, allowing it to be incorporated into any pump-probe experiment, eventually characterizing pulses before and after interaction with most sample environments.
The electro-optic (EO) effect is a powerful diagnostic tool for determining the time profile of ultrashort relativistic electron bunches. When a relativistic bunch passes within a few mm of an ...electro-optic crystal, its transient electric field is equivalent to a half-cycle THz pulse passing through the crystal. The induced birefringence can be detected with polarized femtosecond laser pulses. A simulation code has been written in order to understand the faithfulness and the limitations of electron bunch shape reconstruction by EO sampling. The THz pulse and the laser pulse are propagated as wave packets through the EO crystal. Alternatively, the response function method is applied. Using experimental data on the material properties of zinc telluride (ZnTe) and gallium phosphide (GaP), the effects of velocity mismatch, pulse shape distortion, and signal broadening are explicitly taken into account. The simulations show that the most severe limitation on the time resolution is given by the transverse-optical (TO) lattice oscillation in the EO crystal. The lowest TO frequency is 5.3 THz in ZnTe and 11 THz in GaP. Only the Fourier components below the TO resonance are usable for the bunch shape reconstruction. This implies that the shortest rms bunch length which can be resolved with moderate distortion amounts to σ≈90fs in ZnTe and σ≈50fs in GaP. The influence of the crystal thickness on the amplitude and width of the EO signal is studied. The optimum thickness is in the range from 100 to 300μm for ZnTe and from 50 to 100μm for GaP.
Abstract
The new synchrotron light source PETRA IV at DESY will use a fast orbit feedback system with hundreds of fast corrector magnets to meet stringent orbit stability requirements. These magnets ...are operated at high frequencies, creating strong eddy currents that result in Joule losses and a time delay between applied voltage and aperture field. User experiments impose challenging requirements on beam operation to preserve the point of the radiation source. To meet the demanding feedback requirements, finite element simulations are needed to understand the characteristics of the corrector magnet. However, due to the small skin depths at high frequencies and the laminated structure of the yoke, these simulations need a very fine mesh and are thus very costly. Therefore, we homogenize the laminated yoke which reduces the computational effort but captures the eddy current effects accurately. The reduction of simulation times from several hours to a few minutes allows us to conduct extensive studies of the eddy current losses and the field quality of the magnets.
Clocking Auger electrons Haynes, D. C.; Wurzer, M.; Schletter, A. ...
Nature physics,
04/2021, Letnik:
17, Številka:
4
Journal Article
Recenzirano
Odprti dostop
Intense X-ray free-electron lasers (XFELs) can rapidly excite matter, leaving it in inherently unstable states that decay on femtosecond timescales. The relaxation occurs primarily via Auger ...emission, so excited-state observations are constrained by Auger decay. In situ measurement of this process is therefore crucial, yet it has thus far remained elusive in XFELs owing to inherent timing and phase jitter, which can be orders of magnitude larger than the timescale of Auger decay. Here we develop an approach termed ‘self-referenced attosecond streaking’ that provides subfemtosecond resolution in spite of jitter, enabling time-domain measurement of the delay between photoemission and Auger emission in atomic neon excited by intense, femtosecond pulses from an XFEL. Using a fully quantum-mechanical description that treats the ionization, core-hole formation and Auger emission as a single process, the observed delay yields an Auger decay lifetime of 2.2−0.3+0.2 fs for the KLL decay channel.Self-referenced attosecond streaking enables in situ measurements of Auger emission in atomic neon excited by femtosecond pulses from an X-ray free-electron laser with subfemtosecond time resolution and despite the jitter inherent to X-ray free-electron lasers.
Initiating the gain process in a free-electron laser (FEL) from an external highly coherent source of radiation is a promising way to improve the pulse properties such as temporal coherence and ...synchronization performance in time-resolved pump-probe experiments at FEL facilities, but this so-called "seeding" suffers from the lack of adequate sources at short wavelengths. We report on the first successful seeding at a wavelength as short as 38.2 nm, resulting in GW-level, coherent FEL radiation pulses at this wavelength as well as significant second harmonic emission at 19.1 nm. The external seed pulses are about 1 order of magnitude shorter compared to previous experiments allowing an ultimate time resolution for the investigation of dynamic processes enabling breakthroughs in ultrafast science with FELs. The seeding pulse is the 21st harmonic of an 800-nm, 15-fs (rms) laser pulse generated in an argon medium. Methods for finding the overlap of seed pulses with electron bunches in spatial, longitudinal, and spectral dimensions are discussed and results are presented. The experiment was conducted at FLASH, the FEL user facility at DESY in Hamburg, Germany.
The longitudinal profiles of ultrashort relativistic electron bunches at the soft x-ray free-electron laser FLASH have been investigated using two single-shot detection schemes: an electro-optic (EO) ...detector measuring the Coulomb field of the bunch and a radio-frequency structure transforming the charge distribution into a transverse streak. A comparison permits an absolute calibration of the EO technique. EO signals as short as 60 fs (rms) have been observed, which is a new record in the EO detection of single electron bunches and close to the limit given by the EO material properties.
This paper describes some achievements of the low-level radio frequency (LLRF) tests performed to evaluate the superconducting cryomodules in preparation of their installation in the European X-ray ...Free Electron Laser (XFEL) accelerator. The software developed to characterize the cryomodules tested at the Accelerator Module Test Facility (AMTF) will be presented. The purpose of these tests is to evaluate some of the key parameters of the eight Tera Electronvolt Superconducting Linear Accelerator cavities, housed in every cryomodule. These parameters include: cavity quench gradients, cavity fundamental resonant modes, performance of the slow and fast frequency tuners, and characteristics of the input power coupler. These results impact the final decision on the cryomodule acceptance and its installation inside the linear accelerator (linac). In this approach, the MicroTCA.4-based LLRF system is used to control and assess the cryomodule performance. Middle layer servers are developed to verify the tests initial conditions, carry the test, and log the results in a dedicated database. The tests results provide a basis for the cryomodule validation, but also serve as a reference useful during the commissioning and operating phase of the accelerator.
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