The aerosol shortwave, direct radiative effects of smoke plumes from Chilean wildfires in 2017 and 2023 were derived from satellite observations in both cloud‐free and cloud scenes. At the top of the ...atmosphere, the aerosol DRE changes sign when aerosol overly clouds or open ocean, confirmed by both measurements and a simulation study. The cloud‐free daily‐mean DRE, computed using an offline radiative transfer model (RTM), was 66 W m−2 in 2023 and 42 W m−2 in 2017, due to absorption by smoke. However, the total radiative effects were larger in 2017 due to a larger plume size compared to 2023. The method presented here provides a new conceptual model to quickly assess the radiative effects of wildfire smoke plumes using satellite measurements and pre‐computed RTM results. The presented estimates are strongly affected by the uncertainty of aerosol optical thickness retrievals from satellite, which can be large in the presence of clouds.
Plain Language Summary
From 30 January to the end of February 2023, central Chile experienced over 400 individual wildfires, consuming over 430,000 ha of native sclerophyllous forests, with 25 fatalities as of 14 February. Wildfires are common in central Chile during dry periods, but seem intensified due to the mega‐drought since 2010. Next to health effects, the smoke from these wildfires has important climatic impacts through the change of solar insolation in the atmosphere: smoke strongly absorbs solar radiation and heats the atmosphere, changing the vertical stability. In this paper, the horizontal and vertical smoke distribution in the atmosphere is presented using satellite observations, and the radiative effects in the atmosphere and at the surface are quantified for the recent fires and as well as for the record‐breaking wildfires in 2017, which were the most devastating in the modern history of central‐Chile. Our results show that the radiative effects of the smoke from the recent wildfires were stronger in magnitude during the first few days, but confined to a smaller area, reducing their overall effect.
Key Points
The radiative effects of the recent 2023 Chilean wildfire smoke plumes are assessed and compared to the 2017 Chilean wildfires smoke plumes
Pre‐computed radiative transfer model results can provide readily available aerosol direct radiative effects in clear‐sky for smoke
Satellite measurements can further improve the aerosol direct effect and direct forcing estimates for both clear sky and cloud scenes
•This article overviews polarimetric observations, their history and expected developments, and resulting aerosol products.•The paper was conceived during the workshop APOLO-2017 held in Hefei, ...China, in October 2017.
Polarimetry is one of the most promising types of remote sensing for improved characterization of atmospheric aerosol. Indeed, aerosol particles constitute a highly variable atmospheric component characterized by a large number of parameters describing particle sizes, morphologies (including shape and internal structure), absorption and scattering properties, amounts, horizontal and vertical distribution, etc. Reliable monitoring of all these parameters is very challenging, and therefore the aerosol effects on climate and environment are considered to be among the most uncertain factors in climate and environmental research. In this regard, observations that provide both the angular distribution of the scattered atmospheric radiation as well as its polarization state at multiple wavelengths covering the UV–SWIR spectral range carry substantial implicit information on the atmospheric composition. Therefore, high expectations in improving aerosol characterization are associated with detailed passive photopolarimetric observations.
The critical need to use space-borne polarimetry for global accurate monitoring of detailed aerosol properties was first articulated in the late 1980s and early 1990s. By now, several orbital instruments have already provided polarization observations from space, and a number of advanced missions are scheduled for launch in the coming years by international and national space agencies. The first and most extensive record of polarimetric imagery was provided by POLDER-I, POLDER-II, and POLDER/PARASOL multi-angle multi-spectral polarization sensors. Polarimetric observations with the POLDER-like design intended for collecting extensive multi-angular multi-spectral measurements will be provided by several instruments, such as the MAI/TG-2, CAPI/TanSat, and DPC/GF-5 sensors recently launched by the Chinese Space Agency. Instruments such as the 3MI/MetOp-SG, MAIA, SpexOne and HARP2 on PACE, POSP, SMAC, PCF, DPC–Lidar, ScanPol and MSIP/Aerosol-UA, MAP/Copernicus CO2 Monitoring, etc. are planned to be launched by different space agencies in the coming decade. The concepts of these future instruments, their technical designs, and the accompanying algorithm development have been tested intensively and analyzed using diverse airborne prototypes. Certain polarimetric capabilities have also been implemented in such satellite sensors as GOME-2/MetOp and SGLI/GCOM-C.
A number of aerosol retrieval products have been developed based on the available measurements and successfully used for different scientific applications. However, the completeness and accuracy of aerosol data operationally derived from polarimetry do not yet appear to have reached the accuracy levels implied by theoretical sensitivity studies that analyzed the potential information content of satellite polarimetry. As a result, the dataset provided by MODIS is still most frequently used by the scientific community, yet this sensor has neither polarimetric nor multi-angular capabilities. Admittedly polarimetric multi-angular observations are highly complex and have extra sensitivities to aerosol particle morphology, vertical variability of aerosol properties, polarization of surface reflectance, etc. As such, they necessitate state-of-the-art forward modeling based on first-principles physics which remains rare, and conventional retrieval approaches based on look-up tables turn out to be unsuitable to fully exploit the information implicit in the measurements. Several new-generation retrieval approaches have recently been proposed to address these challenges. These methods use improved forward modeling of atmospheric (polarized) radiances and implement a search in the continuous space of solutions using rigorous statistically optimized inversions. Such techniques provide more accurate retrievals of the main aerosol parameters such as aerosol optical thickness and yield additional parameters such as aerosol absorption. However, the operational implementation of advanced retrieval approaches generally requires a significant extra effort, and the forward-modeling part of such retrievals still needs to be substantially improved.
Ground-based passive polarimetric measurements have also been evolving over the past decade. Although polarimetry helps improve aerosol characterization, especially of the fine aerosol mode, the operators of major observational networks such as AERONET remain reluctant to include polarimetric measurements as part of routine retrievals owing to their high complexity and notable increase in effort required to acquire and interpret polarization data.
In addition to remote-sensing observations, polarimetric characteristics of aerosol scattering have been measured in situ as well as in the laboratory using polar nephelometers. Such measurements constitute direct observations of single scattering with no contributions from multiple scattering effects and therefore provide unique data for the validation of aerosol optical models and retrieval concepts.
This article overviews the above-mentioned polarimetric observations, their history and expected developments, and the state of resulting aerosol products. It also discusses the main achievements and challenges in the exploitation of polarimetry for the improved characterization of atmospheric aerosols.
This study presents an analysis of TROPOMI cloud heights as a proxy for volcanic plume heights in the presence of absorbing aerosols and sulfur dioxide for the 19 February 2018 eruption plume of the ...Sinabung volcano on Sumatra, Indonesia.
In this paper we introduce the new concept of directionally dependent Lambertian-equivalent reflectivity (DLER) of the Earth's surface retrieved from satellite observations. This surface DLER ...describes Lambertian (isotropic) surface reflection which is extended with a dependence on the satellite viewing geometry. We apply this concept to data of the GOME-2 satellite instruments to create a global database of the reflectivity of the Earth's surface, providing surface DLER for 26 wavelength bands between 328 and 772 nm as a function of the satellite viewing angle via a second-degree polynomial parameterisation. The resolution of the database grid is 0.25.sup." by 0.25.sup.", but the real, intrinsic spatial resolution varies over the grid from 1.0.sup." by 1.0.sup." to 0.5.sup." by 0.5.sup." down to 0.25.sup." by 0.25.sup." by applying dynamic gridding techniques. The database is based on more than 10 years (2007-2018) of GOME-2 data from the MetOp-A and MetOp-B satellites.
In this study we present the retrieval of the column-averaged dry air mole fraction of carbon dioxide (XCO2) from the TanSat observations using the ACOS (Atmospheric CO2 Observations from Space) ...algorithm. The XCO2 product has been validated with collocated ground-based measurements from the Total Carbon Column Observing Network (TCCON) for 2 years of TanSat data from 2017 to 2018. Based on the correlation of the XCO2 error over land with goodness of fit in three spectral bands at 0.76, 1.61 and 2.06 μm, we applied an a posteriori bias correction to TanSat retrievals. For overpass averaged results, XCO2 retrievals show a standard deviation (SD) of ~2.45 ppm and a positive bias of ~0.27 ppm compared to collocated TCCON sites. The validation also shows a relatively higher positive bias and variance against TCCON over high-latitude regions. Three cases to evaluate TanSat target mode retrievals are investigated, including one field campaign at Dunhuang with measurements by a greenhouse gas analyzer deployed on an unmanned aerial vehicle and two cases with measurements by a ground-based Fourier-transform spectrometer in Beijing. The results show the retrievals of all footprints, except footprint-6, have relatively low bias (within ~2 ppm). In addition, the orbital XCO2 distributions over Australia and Northeast China between TanSat and the second Orbiting Carbon Observatory (OCO-2) on 20 April 2017 are compared. It shows that the mean XCO2 from TanSat is slightly lower than that of OCO-2 with an average difference of ~0.85 ppm. A reasonable agreement in XCO2 distribution is found over Australia and Northeast China between TanSat and OCO-2.
Abstract Clouds affected by solar eclipses could influence the reflection of sunlight back into space and might change local precipitation patterns. Satellite cloud retrievals have so far not taken ...into account the lunar shadow, hindering a reliable spaceborne assessment of the eclipse-induced cloud evolution. Here we use satellite cloud measurements during three solar eclipses between 2005 and 2016 that have been corrected for the partial lunar shadow together with large-eddy simulations to analyze the eclipse-induced cloud evolution. Our corrected data reveal that, over cooling land surfaces, shallow cumulus clouds start to disappear at very small solar obscurations (~15%). Our simulations explain that the cloud response was delayed and was initiated at even smaller solar obscurations. We demonstrate that neglecting the disappearance of clouds during a solar eclipse could lead to a considerable overestimation of the eclipse-related reduction of net incoming solar radiation. These findings should spur cloud model simulations of the direct consequences of sunlight-intercepting geoengineering proposals, for which our results serve as a unique benchmark.
In this paper a clear‐sky shortwave closure analysis is presented for the Baseline Surface Radiation Network (BSRN) site of Cabauw, Netherlands (51.97°N, 4.93°E). The analysis is based on an ...exceptional period of fine weather during the first half of May 2008, resulting in a selection of 72 comparisons, on 6 days, between BSRN measurements and Doubling Adding KNMI (DAK) model simulations of direct, diffuse, and global irradiances. The data span a wide range of aerosol properties, water vapor columns, and solar zenith angles. The model input consisted of operational Aerosol Robotic Network (AERONET) aerosol products and radiosonde data. The wavelength dependence of the aerosol optical thickness, single scattering albedo, and asymmetry parameter was taken into account. On the basis of these data, excellent closure was obtained: the mean differences between model and measurements are 2 W/m2 (+0.2%) for the direct irradiance, 1 W/m2 (+0.8%) for the diffuse irradiance, and 2 W/m2 (+0.3%) for the global irradiance. The good results were obtained because of proper specification of the DAK model input and the high quality of the AERONET and BSRN measurements. The sensitivity of the achieved closure to uncertainties in the aerosol optical thickness, single scattering albedo, and asymmetry parameter was examined. Furthermore, several sensitivity experiments related to the wavelength dependence of the aerosol optical properties and the treatment of water vapor were performed. It appeared that a correct description of the wavelength dependence of the aerosol optical properties is important for achieving broadband closure. However, broadband closure can also be obtained by means of using spectrally averaged values of the single scattering albedo and the asymmetry parameter. Cancellation of errors in different parts of the solar spectrum also contributes to the achieved closure.
The vulnerability of the (European) aviation system to the airborne hazards was evident during the Eyjafjallajökull volcanic eruption in 2010. For support of Air Traffic Control (ATC) many ...observations of the event were available from satellites, ground based instruments and airborne platforms, at pan-European scale. However, efficient use of the data for ATC proved difficult mainly due to sub-optimal aggregation and integrated assessment of the available information in near-real-time.
The project EUNADICS-AV (European Natural Disaster Coordination and Information System for Aviation) aims to close this gap. The observational component of the project will make existing data products for airborne hazards more accessible, visible and used, and to foster tailored product development. Once assimilated into models and integrated in the EUNADICS-AV Data Portal these data can be the base to efficiently improve European airspace resilience to airborne hazards.
Since 2010 new data products have become available specifically for for airborne hazard alerting and monitoring together with specific tailored products designed for replying to user needs and recommendations.
This paper describes the EUNADICS-AV approach and will focus on the role of operational and research grade ground based lidars.
A radiative transfer model for studying spectral and broadband snow surface albedo has been applied to radiation data (1998–2001) from different climate regimes in Antarctica. The model makes use of ...the doubling‐adding method for radiative transfer, combined with the correlated k‐distribution technique to account for atmospheric gas absorption. Snow layers are described by scattering phase functions for irregular hexagonal plate‐shaped ice crystals. Multiple scattering is included, as well as the option to include soot in the snowpack, as well as clouds. Sensitivity experiments show that the model is capable of calculating spectral and broadband albedos as a function of solar zenith angle and effective snow grain radius re. The novel approach of applying the model to multiple‐year field data of clear‐sky albedo from five locations in Dronning Maud Land, Antarctica, reveals that seasonal clear‐sky albedo variations (0.77–0.88) are dominantly caused by strong spatial and temporal variations in re. Summer season averages of re range from 22 μm on the Antarctic plateau to 64 μm on the ice shelf. Maximum monthly values of re are 40–150% higher. Other factors influencing clear‐sky broadband albedo are the seasonal cycle in solar zenith angle (at most 0.02 difference in summer and spring/autumn albedo) and the spatial variation in optical thickness of the cloudless atmosphere (0.01 difference between ice shelves and plateau). The seasonal cycle in optical thickness of the atmosphere was found to be of minor importance (<0.005 between summer and spring/autumn).
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