Strong coupling in hybrid metal-dielectric nanoresonators Decker, M.; Pertsch, T.; Staude, I.
Philosophical transactions of the Royal Society of London. Series A: Mathematical, physical, and engineering sciences,
03/2017, Letnik:
375, Številka:
2090
Journal Article
Recenzirano
Odprti dostop
We study resonant photonic-plasmonic coupling between a gold dipole nanoantenna and a silicon nanodisc supporting electric and magnetic dipolar Mie-type resonances. Specifically, we consider two ...different cases for the mode structure of the silicon nanodisc, namely spectrally separate and spectrally matching electric and magnetic dipolar Mie-type resonances. In the latter case, the dielectric nanoparticle scatters the far fields of a unidirectional Huygens' source. Our results reveal an anticrossing of the plasmonic dipole resonance and the magnetic Mie-type dipole resonance of the silicon nanodisc, accompanied by a clear signature of photonic-plasmonic mode hybridization in the corresponding mode profiles. These characteristics show that strong coupling is established between the two different resonant systems in the hybrid nanostructure. Furthermore, our results demonstrate that in comparison with purely metallic or dielectric nanostructures, hybrid metal-dielectric nanoresonators offer higher flexibility in tailoring the fractions of light which are transmitted, absorbed and reflected by the nanostructure over a broad range of parameters without changing its material composition. As a special case, highly asymmetric reflection and absorption properties can be achieved.
This article is part of the themed issue ‘New horizons for nanophotonics’.
Light interaction with disordered materials is both complex and fascinating at the same time. Here, we reveal disorder-induced phase transitions in a dielectric Huygens' metasurface made from silicon ...nanocylinders that simultaneously support an electric and magnetic dipole resonance. Depending on the degree of positional disorder and the spectral detuning of the two resonances, the phase angle of the transmission coefficient exhibits a clear phase transition from normal to anomalous dispersion. Combined with the considerations of whether the resonances of spectrally detuned particles appear as separated or overlapping, we distinguish four different phase states. We study this phenomenon analytically by employing dipole particles and disclose the entire phase diagram, support our insights with full-wave simulations of actual structures, and corroborate the findings with experimental results. Unveiling this phenomenon is a milestone simultaneously in the growing fields of metamaterial-inspired silicon nanophotonics, photonics in disordered media, and the fundamental physics of phase transitions.
Abstract
Monolayer transition metal dichalcogenides (TMD) have numerous potential applications in ultrathin electronics and photonics. The exposure of TMD-based devices to light generates ...photo-carriers resulting in an enhanced conductivity, which can be effectively used, e.g., in photodetectors. If the photo-enhanced conductivity persists after removal of the irradiation, the effect is known as persistent photoconductivity (PPC). Here we show that ultraviolet light (λ = 365 nm) exposure induces an extremely long-living giant PPC (GPPC) in monolayer MoS
2
(ML-MoS
2
) field-effect transistors (FET) with a time constant of ~30 days. Furthermore, this effect leads to a large enhancement of the conductivity up to a factor of 10
7
. In contrast to previous studies in which the origin of the PPC was attributed to extrinsic reasons such as trapped charges in the substrate or adsorbates, we show that the GPPC arises mainly from the intrinsic properties of ML-MoS
2
such as lattice defects that induce a large number of localized states in the forbidden gap. This finding is supported by a detailed experimental and theoretical study of the electric transport in TMD based FETs as well as by characterization of ML-MoS
2
with scanning tunneling spectroscopy, high-resolution transmission electron microscopy, and photoluminescence measurements. The obtained results provide a basis for the defect-based engineering of the electronic and optical properties of TMDs for device applications.
We perform multipolar analysis of second-harmonic generation (SHG) from (111)-grown gallium arsenide (GaAs) nanoantennas and discuss its specifics. It was experimentally demonstrated that the ...conversion efficiency in axially-symmetric (111) GaAs nanoparticles remains constant under the polarization rotation of normally incident radiation in a wide range of particle sizes, while the SHG radiation pattern changes. We apply the analytical method based on the Lorentz lemma to explain this behaviour. The induced nonlinear current is decomposed into two rotating contributions, which are shown to generate multipoles of different parities. Thus, the total SHG intensity in the far-field is proved to be independent of the in-plane rotation of the pump polarization. Nevertheless, due to the threefold symmetry of the crystal with regard to the (111) direction, the SHG radiation pattern rotates around the polar axis repeating its shape every 60°.
•A hybrid metal-dielectric antenna boosted the performance of single-photon sources.•A gold dimer constituted by cylinders provided large Purcell factor values.•Quadrupolar electric resonance ...excitation in the gold dimer provided directionality.•Silicon directors further improved the directivity.
The confinement of electromagnetic energy to subwavelength volumes through nanoscale antennas can be used to enhance the spontaneous emission of quantum emitters. With this aim, different configurations of metallic and high refractive index dielectric nanoparticles have been explored. Here, we carry out a comparative analysis of planar metallic, high refractive index dielectric, and hybrid nanoantennas considering three different parameters: the Purcell factor enhancement, radiation efficiency, and directionality properties. We focus our study on different geometries and material combinations of a dimer of cylinders. A dimer made of two gold nanocylinders is the most promising candidate for improving the spontaneous emission. While most previous works have paid attention to the redirection of the scattered emission in the nanoparticle plane, our proposed nanostructure of two large gold cylinders (R=λ/4) emits most of the radiation upwards. This effect is due to the strong quadrupolar electric contribution to the resonant mode. With the aim to further improve the directionality properties, additional silicon nanocylinders are used as directors of the scattered radiation, increasing the directivity by a factor of 2.4 with respect to the gold dimer without directors. All in all, a hybrid structure composed of a gold dimer and silicon nanoparticles is proposed to enhance the spontaneous emission of a single quantum dot and to govern its emission pattern. The results shown in this work could be useful in fluorescence enhancement or in quantum photonics. They are particularly interesting for the development of single-photon sources based on quantum dots and other nanoscale emitters.
Strong coupling in hybrid metal–dielectric nanoresonators Decker, M.; Pertsch, T.; Staude, I.
Philosophical transactions of the Royal Society of London. Series A: Mathematical, physical, and engineering sciences,
03/2017, Letnik:
375, Številka:
2090
Journal Article
Recenzirano
We study resonant photonic–plasmonic coupling between a gold dipole nanoantenna and a silicon nanodisc supporting electric and magnetic dipolar Mie-type resonances. Specifically, we consider two ...different cases for the mode structure of the silicon nanodisc, namely spectrally separate and spectrally matching electric and magnetic dipolar Mie-type resonances. In the latter case, the dielectric nanoparticle scatters the far fields of a unidirectional Huygens' source. Our results reveal an anticrossing of the plasmonic dipole resonance and the magnetic Mie-type dipole resonance of the silicon nanodisc, accompanied by a clear signature of photonic–plasmonic mode hybridization in the corresponding mode profiles. These characteristics show that strong coupling is established between the two different resonant systems in the hybrid nanostructure. Furthermore, our results demonstrate that in comparison with purely metallic or dielectric nanostructures, hybrid metal–dielectric nanoresonators offer higher flexibility in tailoring the fractions of light which are transmitted, absorbed and reflected by the nanostructure over a broad range of parameters without changing its material composition. As a special case, highly asymmetric reflection and absorption properties can be achieved. This article is part of the themed issue 'New horizons for nanophotonics'.
Recent progress in three-dimensional sub-micron fabrication has rendered the introduction of waveguide structures into optical three-dimensional photonic bandgap materials possible. However, spectral ...tuning of the waveguide modes has not been demonstrated so far. Here, we use atomic-layer deposition of amorphous silica to tune the spectral position of an air-core defect waveguide in a three-dimensional silicon woodpile photonic crystal by 225 nm in wavelength. The measured spectral positions of the waveguide signature are in very good agreement with numerical calculations.
Probing plasmonic electro-magnetic environment with Eu3 Noginova, N.; Hussain, R.; Noginov, M. A. ...
2014 Conference on Lasers and Electro-Optics (CLEO) - Laser Science to Photonic Applications,
2014-June
Conference Proceeding
We use spontaneous emission of Eu 3+ ions as a spectroscopic tool to probe modifications of optical fields in close vicinity of metal and under the conditions of the optically-induced magnetic ...resonance. We reveal strictly different behavior of electric and magnetic dipole emission in a simple microscope setup, and also discuss the results theoretically.
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