Offsets between the primary and secondary coils of loosely coupled transformers (LCT) are attributable to the efficiency decline of the wireless power transfer (WPT) system. To improve the misalignment tolerance of efficiency in WPT system, this paper presents a LCT system with a movable intermediate coil and adjustable system frequency, which can promote the efficiency of the WPT system under misalignment condition. First, the influences of the position and compensation parameter of intermediate coil on the system efficiency during migration are summarized. The optimal compensation parameter and optimal position selection method of intermediate coil are proposed. Then, the influence of frequency on system efficiency is studied, and the detailed control strategy of intermediate coil's position and system frequency is proposed. A 3-kW prototype WPT with the proposed three-coil LCT is manufactured and experimental validations are also performed. The results show that the efficiency declines of three-coil LCT with the proposed control strategy is 1.8% when the lateral offsets reach 300mm, namely 43% of the outer diameter of coil.