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Chang, Jeong Ah; Rhee, Jae Hui; Im, Sang Hyuk; Lee, Yong Hui; Kim, Hi-jung; Seok, Sang Il; Nazeeruddin, Md. K; Gratzel, Michael
Nano letters, 2010-Jul-14, Letnik: 10, Številka: 7Journal Article
We report all solid-state nanostructured inorganic−organic heterojunction solar cells fabricated by depositing Sb2S3 and poly(3-hexylthiophene) (P3HT) on the surface of a mesoporous TiO2 layer, where Sb2S3 acts as an absorbing semiconductor and P3HT acts as both a hole conductor and light absorber. These inorganic−organic light harvesters perform remarkably well with a maximum incident-photon-to-current efficiency (IPCE) of 80% and power conversion efficiency of 5.13% under air-mass 1.5 global (AM 1.5G) illumination with the intensity of 100 mW cm−2. These devices are highly stable under room light in air, even without encapsulation. The present findings offer novel directions for achieving high-efficiency solid-state solar cells by hybridization of inorganic−organic light harvesters and hole transporters.
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