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Schultze, M; Fiess, M; Karpowicz, N; Gagnon, J; Korbman, M; Hofstetter, M; Neppl, S; Cavalieri, A.L; Komninos, Y; Mercouris, Th; Nicolaides, C.A; Pazourek, R; Nagele, S; Feist, J; Burgdörfer, J; Azzeer, A.M; Ernstorfer, R; Kienberger, R; Kleineberg, U; Goulielmakis, E; Krausz, F; Yakovlev, V.S
Science, 06/2010, Letnik: 328, Številka: 5986Journal Article
Photoemission from atoms is assumed to occur instantly in response to incident radiation and provides the basis for setting the zero of time in clocking atomic-scale electron motion. We used attosecond metrology to reveal a delay of Formula: see text attoseconds in the emission of electrons liberated from the 2p orbitals of neon atoms with respect to those released from the 2s orbital by the same 100-electron volt light pulse. Small differences in the timing of photoemission from different quantum states provide a probe for modeling many-electron dynamics. Theoretical models refined with the help of attosecond timing metrology may provide insight into electron correlations and allow the setting of the zero of time in atomic-scale chronoscopy with a precision of a few attoseconds.
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