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do Carmo, José Vitor C.; Bezerra, Rita de Cássia F.; Tehuacanero-Cuapa, Samuel; Rodríguez-Aguado, E.; Lang, Rossano; Campos, Adriana F.; Duarte, Gian; Saraiva, Gilberto D.; Otubo, Larissa; Oliveira, Alcineia C.; Rodríguez-Castellón, E.
Materials chemistry and physics, 12/2022, Letnik: 292Journal Article
A tailored nanostructured CuO–ZnO/Al2O3 catalyst was obtained from nanocomposites via sonochemical route through core/shell assisted by reverse micelle synthesis. The as-synthesized nanocomposites consisted of Cu, Zn and Al domains coated by a lauric acid shell structure with controlled physicochemical properties. Combining these features, a porous CuO–ZnO/Al2O3 supported catalyst was obtained from CuZnAl@C nanocomposite, in which Cu and Zn oxide nanoparticles interacted quite strongly with alumina. In this study, a nanostructured CuO–ZnO/Al2O3 was applied to oxidize ethylbenzene in the presence of H2O2. Catalytic results further demonstrated that the nanostructured solid had ethylbenzene conversion superior to 20% and good selectivities to acetophenone, benzaldehyde and benzoic acid compared to a benchmark CuZnAl catalyst obtained by the sol-gel method. Display omitted •Tailored CuO–ZnO/Al2O3 catalyst obtained from CuZnAl@C nanocomposite.•Simple sonochemical route via core/shell assisted by reverse micelle synthesis.•Nuclei composed of Cu and Zn domains coated by a semi-crystalline lauric acid-based shell.•Highly dispersed CuO and ZnO on alumina converting ehtylbenzene.
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Leto | Faktor vpliva | Izdaja | Kategorija | Razvrstitev | ||||
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JCR | SNIP | JCR | SNIP | JCR | SNIP | JCR | SNIP |
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in: SICRIS
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