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Chong, Lina; Wen, Jianguo; Kubal, Joseph; Sen, Fatih G; Zou, Jianxin; Greeley, Jeffery; Chan, Maria; Barkholtz, Heather; Ding, Wenjiang; Liu, Di-Jia
Science (American Association for the Advancement of Science), 12/2018, Letnik: 362, Številka: 6420Journal Article
Achieving high catalytic performance with the lowest possible amount of platinum is critical for fuel cell cost reduction. Here we describe a method of preparing highly active yet stable electrocatalysts containing ultralow-loading platinum content by using cobalt or bimetallic cobalt and zinc zeolitic imidazolate frameworks as precursors. Synergistic catalysis between strained platinum-cobalt core-shell nanoparticles over a platinum-group metal (PGM)-free catalytic substrate led to excellent fuel cell performance under 1 atmosphere of O or air at both high-voltage and high-current domains. Two catalysts achieved oxygen reduction reaction (ORR) mass activities of 1.08 amperes per milligram of platinum (A mg ) and 1.77 A mg and retained 64% and 15% of initial values after 30,000 voltage cycles in a fuel cell. Computational modeling reveals that the interaction between platinum-cobalt nanoparticles and PGM-free sites improves ORR activity and durability.
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