E-viri
Recenzirano
Odprti dostop
-
Akri, Mohcin; Zhao, Shu; Li, Xiaoyu; Zang, Ketao; Lee, Adam F; Isaacs, Mark A; Xi, Wei; Gangarajula, Yuvaraj; Luo, Jun; Ren, Yujing; Cui, Yi-Tao; Li, Lei; Su, Yang; Pan, Xiaoli; Wen, Wu; Pan, Yang; Wilson, Karen; Li, Lin; Qiao, Botao; Ishii, Hirofumi; Liao, Yen-Fa; Wang, Aiqin; Wang, Xiaodong; Zhang, Tao
Nature communications, 11/2019, Letnik: 10, Številka: 1Journal Article
Dry reforming of methane (DRM) is an attractive route to utilize CO as a chemical feedstock with which to convert CH into valuable syngas and simultaneously mitigate both greenhouse gases. Ni-based DRM catalysts are promising due to their high activity and low cost, but suffer from poor stability due to coke formation which has hindered their commercialization. Herein, we report that atomically dispersed Ni single atoms, stabilized by interaction with Ce-doped hydroxyapatite, are highly active and coke-resistant catalytic sites for DRM. Experimental and computational studies reveal that isolated Ni atoms are intrinsically coke-resistant due to their unique ability to only activate the first C-H bond in CH , thus avoiding methane deep decomposition into carbon. This discovery offers new opportunities to develop large-scale DRM processes using earth abundant catalysts.
Avtor
Vnos na polico
Trajna povezava
- URL:
Faktor vpliva
Dostop do baze podatkov JCR je dovoljen samo uporabnikom iz Slovenije. Vaš trenutni IP-naslov ni na seznamu dovoljenih za dostop, zato je potrebna avtentikacija z ustreznim računom AAI.
Leto | Faktor vpliva | Izdaja | Kategorija | Razvrstitev | ||||
---|---|---|---|---|---|---|---|---|
JCR | SNIP | JCR | SNIP | JCR | SNIP | JCR | SNIP |
Baze podatkov, v katerih je revija indeksirana
Ime baze podatkov | Področje | Leto |
---|
Povezave do osebnih bibliografij avtorjev | Povezave do podatkov o raziskovalcih v sistemu SICRIS |
---|
Vir: Osebne bibliografije
in: SICRIS
To gradivo vam je dostopno v celotnem besedilu. Če kljub temu želite naročiti gradivo, kliknite gumb Nadaljuj.