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Chemical diffusion through grain boundaries in mixed conductorsJamnik, Janko ; Maier, JoachimChemical diffusion through boudaries involving two charged diffusing species (e.g., O[sup](2-) and 2e[sup]- in an oxide) is modeled taking into account Poisson's equation, restricted to dilute ... systems and small driving forces. Theresults are compared with conventional treatments on a single crystal. Grain boundary effects are exemplified for (i) a bicrystal containing a grain boundary with adjacent space-charge layers and (ii) a polycrystal involving space-charge-free amorphous grain boudaries. Numerical results (i) are analysed in the context of recent experiments on a SrTiO[sub]3 bicrystal. Transmission-line approximations for chemical diffusion in polycrystals are proposed and briefly compared with exact results.Source: Journal of the Electrochemical Society. - ISSN 0013-4651 (Vol. 145, no. 5, 1998, str. 1762-1767)Type of material - article, component partPublish date - 1998Language - englishCOBISS.SI-ID - 1662490
Author
Jamnik, Janko |
Maier, Joachim
Topics
difuzija |
kemijska |
zrna |
meje med zrni |
prostorski naboj |
stroncijev titanat |
SrTiO3 |
bikristal |
polikristal |
diffusion |
chemical |
grains |
grain boundary |
space charge |
strontium titanate |
SrTiO3 |
bycrystal |
polycrystal
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source: Journal of the Electrochemical Society. - ISSN 0013-4651 (Vol. 145, no. 5, 1998, str. 1762-1767)
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Jamnik, Janko | 10180 |
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