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Ba[sub]4[Mn[sub]3N[sub]6], a quasi-one-dimensional mixed-valent nitridomanganate (II, IV)Ovchinnikov, A. ...The mixed-valent nitridomanganate Ba4[Mn3N6] was prepared using a gas%solid high temperature route. The crystal structure was determined employing high resolution synchrotron powder diffraction data: ... space group Pbcn, a = 9.9930(1) Å, b = 6.17126(8) Å, c = 14.4692(2) Å, V = 892.31(2) Å3, Z = 4. The manganese atoms in the structure of Ba4[Mn3N6] are four-fold coordinated by nitrogen forming infinite corrugated chains of edge-sharing [MnN4] tetrahedra. The chains demonstrate a complete charge order of Mn species. Magnetization measurements and first principle calculations indicate quasi-one dimensional magnetic behavior. In addition, chemical bonding analysis revealed pronounced Mn%Mn interactions along the chains.Source: Crystals [Elektronski vir]. - ISSN 2073-4352 (Iss. 6, Vol. 8, 2018)Type of material - e-articlePublish date - 2018Language - englishCOBISS.SI-ID - 33128743
Author
Ovchinnikov, A. |
Bobnar, Matej |
Prots, Yurii |
Schnelle, W. |
Höhn, Peter |
Grin, Yuri
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fizika trdne snovi
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Database name | Field | Year |
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Ovchinnikov, A. | ![]() |
Bobnar, Matej | 29518 |
Prots, Yurii | ![]() |
Schnelle, W. | ![]() |
Höhn, Peter | ![]() |
Grin, Yuri | ![]() |
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