Photoredox Catalysis: The Need to Elucidate the Photochemical Mechanism

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Photoredox Catalysis: The Need to Elucidate the Photochemical Mechanism

Marchini, Marianna; Bergamini, Giacomo; Cozzi, Pier Giorgio; Ceroni, Paola; Balzani, Vincenzo

Angewandte Chemie International Edition, October 9, 2017, Volume: 56, Issue: 42

Journal Article

The photocatalytic mechanism reported in a recent Communication to produce the radical anion of pyrenes postulates a highly endergonic electron transfer process. An analysis of the thermodynamics is reported together with the proposal of an alternative thermodynamically feasible mechanism.

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Marchini, Marianna | Bergamini, Giacomo | Cozzi, Pier Giorgio | Ceroni, Paola | Balzani, Vincenzo

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