Satellite quantification of aerosol effects on clouds relies on
aerosol optical depth (AOD) as a proxy for aerosol concentration or cloud
condensation nuclei (CCN). However, the lack of error ...characterization of
satellite-based results hampers their use for the evaluation and improvement
of global climate models. We show that the use of AOD for assessing
aerosol–cloud interactions (ACIs) is inadequate over vast oceanic areas in
the subtropics. Instead, we postulate that a more physical approach that
consists of matching vertically resolved aerosol data from the Cloud-Aerosol
Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellite at
the cloud-layer height with Moderate Resolution Imaging
Spectroradiometer (MODIS) Aqua cloud retrievals reduces uncertainties in
satellite-based ACI estimates. Combined aerosol extinction coefficients
(σ) below cloud top (σBC) from the Cloud-Aerosol Lidar
with Orthogonal Polarization (CALIOP) and cloud droplet number
concentrations (Nd) from MODIS Aqua yield high correlations across a
broad range of σBC values, with σBC quartile
correlations ≥0.78. In contrast, CALIOP-based AOD yields correlations
with MODIS Nd of 0.54–0.62 for the two lower AOD quartiles. Moreover,
σBC explains 41 % of the spatial variance in MODIS Nd,
whereas AOD only explains 17 %, primarily caused by the lack of spatial
covariability in the eastern Pacific. Compared with σBC,
near-surface σ weakly correlates in space with MODIS Nd,
accounting for a 16 % variance. It is concluded that the linear regression
calculated from ln(Nd)–ln(σBC) (the standard method for
quantifying ACIs) is more physically meaningful than that derived from the
Nd–AOD pair.
Forest ecosystems store approximately 45% of the carbon found in terrestrial ecosystems, but they are sensitive to climate-induced dieback. Forest die-off constitutes a large uncertainty in ...projections of climate impacts on terrestrial ecosystems, climate–ecosystem interactions, and carbon-cycle feedbacks. Current understanding of the physiological mechanisms mediating climate-induced forest mortality limits the ability to model or project these threshold events. We report here a direct and in situ study of the mechanisms underlying recent widespread and climate-induced trembling aspen (Populus tremuloides) forest mortality in western North America. We find substantial evidence of hydraulic failure of roots and branches linked to landscape patterns of canopy and root mortality in this species. On the contrary, we find no evidence that drought stress led to depletion of carbohydrate reserves. Our results illuminate proximate mechanisms underpinning recent aspen forest mortality and provide guidance for understanding and projecting forest die-offs under climate change.
The algorithm to produce the Clouds and the Earth’s Radiant Energy System (CERES) Edition 4.0 (Ed4) Energy Balanced and Filled (EBAF)-surface data product is explained. The algorithm forces computed ...top-of-atmosphere (TOA) irradiances to match with Ed4 EBAF-TOA irradiances by adjusting surface, cloud, and atmospheric properties. Surface irradiances are subsequently adjusted using radiative kernels. The adjustment process is composed of two parts: bias correction and Lagrange multiplier. The bias in temperature and specific humidity between 200 and 500 hPa used for the irradiance computation is corrected based on observations by Atmospheric Infrared Sounder (AIRS). Similarly, the bias in the cloud fraction is corrected based on observations by Cloud–Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) and CloudSat. Remaining errors in surface, cloud, and atmospheric properties are corrected in the Lagrange multiplier process. Ed4 global annual mean (January 2005 through December 2014) surface net shortwave (SW) and longwave (LW) irradiances increase by 1.3 W m−2 and decrease by 0.2 W m−2, respectively, compared to EBAF Edition 2.8 (Ed2.8) counterparts (the previous version), resulting in an increase in net SW + LW surface irradiance of 1.1 W m−2. The uncertainty in surface irradiances over ocean, land, and polar regions at various spatial scales are estimated. The uncertainties in all-sky global annual mean upward and downward shortwave irradiance are 3 and 4 W m−2, respectively, and the uncertainties in upward and downward longwave irradiance are 3 and 6 W m−2, respectively. With an assumption of all errors being independent, the uncertainty in the global annual mean surface LW + SW net irradiance is 8 W m−2.
The radiative effects of the large‐scale air traffic slowdown during April and May 2020 due to the international response to the COVID‐19 pandemic are estimated by comparing the coverage (CC), ...optical properties, and radiative forcing of persistent linear contrails over the conterminous United States and two surrounding oceanic air corridors during the slowdown period and a similar baseline period during 2018 and 2019 when air traffic was unrestricted. The detected CC during the slowdown period decreased by an area‐averaged mean of 41% for the three analysis boxes. The retrieved contrail optical properties were mostly similar for both periods. Total shortwave contrail radiative forcings (CRFs) during the slowdown were 34% and 42% smaller for Terra and Aqua, respectively. The corresponding differences for longwave CRF were 33% for Terra and 40% for Aqua. To account for the impact of any changes in the atmospheric environment between baseline and slowdown periods on detected CC amounts, the contrail formation potential (CFP) was computed from reanalysis data. In addition, a filtered CFP (fCFP) was also developed to account for factors that may affect contrail formation and visibility of persistent contrails in satellite imagery. The CFP and fCFP were combined with air traffic data to create empirical models that estimated CC during the baseline and slowdown periods and were compared to the detected CC. The models confirm that decreases in CC and radiative forcing during the slowdown period were mostly due to the reduction in air traffic, and partly due to environmental changes.
Plain Language Summary
Contrails produced by aircraft flying in cold but humid air both warm the atmosphere by reducing infrared radiation emitted back into space and cool it by increasing reflected sunlight. Due to the decrease in air traffic during the first months of the COVID pandemic, fewer satellite‐detectable contrails were produced compared to pre‐pandemic times, and thus the radiative effects of contrails were also diminished. But changes in the overall temperature and humidity at aircraft cruise altitudes also affect contrail formation and might explain at least some of the observed decrease in contrail coverage during April and May 2020. Analysis of satellite imagery showed that the thickness and ice‐crystal size of the contrails during the COVID period did not change much from pre‐pandemic contrails. The regional contrail coverage was accurately simulated from a combination of the estimated air traffic activity at cruise altitude and the probable frequency of when atmospheric conditions were favorable for contrail formation. This simulation confirms that most of the decrease in contrails and their radiative effects during the COVID‐related slowdown period were due to the reduction in air traffic, and to a lesser extent to changes in temperature and humidity at cruise altitude during April and May 2020.
Key Points
Contrail coverage during the start of the COVID pandemic was reduced significantly over the study area, mostly due to less air traffic
Monthly mean coverage was accurately estimated from a simple relation between air traffic and contrail formation probability
The relation confirms that the decrease in contrail radiative effects is greater than that expected from the decrease in air traffic alone
Biomass burning smoke particles, due to their submicron particle size in relation to the average thermal infrared (TIR) wavelength, theoretically have negligible signals at the TIR channels. However, ...nearly instantaneous longwave (LW) signatures of thick smoke plumes can be frequently observed at the TIR channels from remotely sensed data, including at 10.6 µm (IR window), as well as in water-vapor-sensitive wavelengths at 7.3, 6.8, and 6.3 µm (e.g., lower, middle, and upper troposphere). We systematically evaluated multiple hypotheses as to causal factors of these IR signatures of biomass burning smoke using a combination of data from the Aqua MODerate resolution Imaging Spectroradiometer (MODIS), Aqua Cloud and the Earth Radiant Energy System (CERES), Geostationary Operational Environmental Satellite 16/17 (GOES-16/17) Advanced Baseline Imager, and Suomi-NPP Visible Infrared Imaging Radiometer Suite (VIIRS) and Cross-track Infrared Sounder (CrIS). The largely clear transmission of light through wildfire smoke in the near infrared indicates that coarse or giant ash particles are unlikely to be the dominant cause. Rather, clear signals in water vapor and TIR channels suggest that both co-transported water vapor injected to the middle to upper troposphere and surface cooling by the reduction of surface radiation by the plume are more significant, with the surface cooling effect of smoke aloft being the most dominant. Giving consideration of the smoke impacts on TIR and longwave, CERES indicates that large wildfire aerosol plumes are more radiatively neutral. Further, this smoke-induced TIR signal may be used to map very optically thick smoke plumes, where traditional aerosol retrieval methods have difficulties.
Drawbacks of current carbon dioxide capture methods include corrosivity, evaporative losses and fouling. Separating the capture solvent from infrastructure and effluent gases via microencapsulation ...provides possible solutions to these issues. Here we report carbon capture materials that may enable low-cost and energy-efficient capture of carbon dioxide from flue gas. Polymer microcapsules composed of liquid carbonate cores and highly permeable silicone shells are produced by microfluidic assembly. This motif couples the capacity and selectivity of liquid sorbents with high surface area to facilitate rapid and controlled carbon dioxide uptake and release over repeated cycles. While mass transport across the capsule shell is slightly lower relative to neat liquid sorbents, the surface area enhancement gained via encapsulation provides an order-of-magnitude increase in carbon dioxide absorption rates for a given sorbent mass. The microcapsules are stable under typical industrial operating conditions and may be used in supported packing and fluidized beds for large-scale carbon capture.
Genetic alterations that activate NOTCH1 signaling and T cell transcription factors, coupled with inactivation of the INK4/ARF tumor suppressors, are hallmarks of T-lineage acute lymphoblastic ...leukemia (T-ALL), but detailed genome-wide sequencing of large T-ALL cohorts has not been carried out. Using integrated genomic analysis of 264 T-ALL cases, we identified 106 putative driver genes, half of which had not previously been described in childhood T-ALL (for example, CCND3, CTCF, MYB, SMARCA4, ZFP36L2 and MYCN). We describe new mechanisms of coding and noncoding alteration and identify ten recurrently altered pathways, with associations between mutated genes and pathways, and stage or subtype of T-ALL. For example, NRAS/FLT3 mutations were associated with immature T-ALL, JAK3/STAT5B mutations in HOXA1 deregulated ALL, PTPN2 mutations in TLX1 deregulated T-ALL, and PIK3R1/PTEN mutations in TAL1 deregulated ALL, which suggests that different signaling pathways have distinct roles according to maturational stage. This genomic landscape provides a logical framework for the development of faithful genetic models and new therapeutic approaches.
Two photon polymerization (TPP) is a precise, reliable, and increasingly popular technique for rapid prototyping of micro-scale parts with sub-micron resolution. The materials of choice underlying ...this process are predominately acrylic resins cross-linked via free-radical polymerization. Due to the nature of the printing process, the derived parts are only partially cured and the corresponding mechanical properties, i.e. modulus and ultimate strength, are lower than if the material were cross-linked to the maximum extent. Herein, post-print curing via UV-driven radical generation, is demonstrated to increase the overall degree of cross-linking of low density, TPP-derived structures.
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