Green Approach for Visible-Light-Induced Direct Functionalization of 2‑Methylquinolines

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Green Approach for Visible-Light-Induced Direct Functionalization of 2‑Methylquinolines

Dantas, Juliana A; Echemendía, Radell; Santos, Marilia S; Paixão, Márcio W; Ferreira, Marco Antonio B; Corrêa, Arlene G

Journal of organic chemistry, 09/2020, Volume: 85, Issue: 18

Journal Article

A transition metal- and oxidant-free visible light-photoinduced protocol for direct functionalization of 2-methylquinolines has been developed. This protocol enabled the C–H functionalization of substituted 2-methylquinolines with diacetyl or ethyl pyruvate, under environmentally friendly conditions. A mechanistic investigation based on density functional theory (DFT) calculations provided details about the origins of reactivity and selectivity.

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