Rh(I)-catalyzed asymmetric transfer hydrogenation of α-enamidophosphonates to α-aminophosphonates

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Rh(I)-catalyzed asymmetric transfer hydrogenation of α-enamidophosphonates to α-aminophosphonates

Feng, Yuting; Viereck, Peter; Li, Shi-Guang; Tsantrizos, Youla S.

Tetrahedron, 08/2022, Volume: 121

Journal Article

An asymmetric Rh-catalyzed transfer hydrogenation was developed for the conversion of α-enamidophosphonates to α-aminophosphonates (α-APs) using isopropanol as the hydride donor. This methodology is amenable to a broad substrate scope. A library of structurally diverse α-APs was synthesized in moderate to good yield and enantiomeric excess, having a methylene moiety at Cβ and aryl, heteroaryl or alkyl side chains. Display omitted

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Feng, Yuting | Viereck, Peter | Li, Shi-Guang | Tsantrizos, Youla S.

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