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Ren, Zekun; Oviedo, Felipe; Thway, Muang; Tian, Siyu I P; Wang, Yue; Xue, Hansong; Perea, Jose Dario; Layurova, Mariya; Heumueller, Thomas; Birgersson, Erik; Aberle, Armin; Brabec, Christoph J; Stangl, Rolf; Sun, Shijing; Li, Qianxiao; Lin, Fen; Peters, Ian Marius; Buonassisi, Tonio
arXiv (Cornell University), 11/2019Paper, Journal Article
Process optimization of photovoltaic devices is a time-intensive, trial and error endeavor, without full transparency of the underlying physics, and with user-imposed constraints that may or may not lead to a global optimum. Herein, we demonstrate that embedding physics domain knowledge into a Bayesian network enables an optimization approach that identifies the root cause(s) of underperformance with layer by-layer resolution and reveals alternative optimal process windows beyond global black-box optimization. Our Bayesian-network approach links process conditions to materials descriptors (bulk and interface properties, e.g., bulk lifetime, doping, and surface recombination) and device performance parameters (e.g., cell efficiency), using a Bayesian inference framework with an autoencoder-based surrogate device-physics model that is 100x faster than numerical solvers. With the trained surrogate model, our approach is robust and reduces significantly the time consuming experimentalist intervention, even with small numbers of fabricated samples. To demonstrate our method, we perform layer-by-layer optimization of GaAs solar cells. In a single cycle of learning, we find an improved growth temperature for the GaAs solar cells without any secondary measurements, and demonstrate a 6.5% relative AM1.5G efficiency improvement above baseline and traditional black-box optimization methods.
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