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Potts, Daniel A; Timmis, Roger; Ferranti, Emma J. S; Vande Hey, Joshua D
Atmospheric chemistry and physics, 04/2023, Volume: 23, Issue: 7Journal Article
Recent developments in atmospheric remote sensing from satellites have made it possible to resolve daily emission plumes from industrial point sources around the globe. Wind rotation aggregation coupled with statistical fitting is commonly used to extract emission estimates from these observations. These methods are used here to investigate how the Coriolis effect influences the trajectory of observed emission plumes as well as to assess the impact of this influence on satellite-derived emission estimates. Of the 16 industrial sites investigated, 9 showed the expected curvature for the hemisphere that they reside in, 5 showed no or negligible curvature, and 2 showed opposing or unusual curvature. The sites that showed conflicting curvature reside in topographically diverse regions, where strong meso-γ-scale (2-20 km) turbulence dominates over larger synoptic circulation patterns. For high-curvature cases, the assumption that the wind-rotated plume aggregate is symmetrically distributed across the downwind axis breaks down, which impairs the quality of statistical fitting procedures. Using annual NO.sub.x emissions from Matimba power station as a test case, not compensating for Coriolis curvature resulted in an underestimation of ⼠9 % on average for the years 2018 to 2021. This study is the first formal observation of the Coriolis effect and its influence on satellite-derived emission estimates, and it highlights both the variability in the emission calculation methods and the need for a standardised scheme for these data to act as evidence for regulators.
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