Reduced Graphene Oxide as a Solid-State Electron Mediator in Z-Scheme Photocatalytic Water Splitting under Visible Light

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Reduced Graphene Oxide as a Solid-State Electron Mediator in Z-Scheme Photocatalytic Water Splitting under Visible Light

Iwase, Akihide; Ng, Yun Hau; Ishiguro, Yoshimi; Kudo, Akihiko; Amal, Rose

Journal of the American Chemical Society, 07/2011, Volume: 133, Issue: 29

Journal Article

The effectiveness of reduced graphene oxide as a solid electron mediator for water splitting in the Z-scheme photocatalysis system is demonstrated. We show that a tailor-made, photoreduced graphene oxide can shuttle photogenerated electrons from an O2-evolving photocatalyst (BiVO4) to a H2-evolving photocatalyst (Ru/SrTiO3:Rh), tripling the consumption of electron–hole pairs in the water splitting reaction under visible-light irradiation.

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Iwase, Akihide | Ng, Yun Hau | Ishiguro, Yoshimi | Kudo, Akihiko | Amal, Rose

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