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  • Sea spray aerosol organic e...
    Cravigan, Luke T; Mallet, Marc D; Vaattovaara, Petri; Harvey, Mike J; Law, Cliff S; Modini, Robin L; Russell, Lynn M; Stelcer, Ed; Cohen, David D; Olsen, Greg; Safi, Karl; Burrell, Timothy J; Ristovski, Zoran

    Atmospheric chemistry and physics, 07/2020, Volume: 20, Issue: 13
    Journal Article

    The aerosol-driven radiative effects on marine low-level cloud represent a large uncertainty in climate simulations, in particular over the Southern Ocean, which is also an important region for sea spray aerosol production. Observations of sea spray aerosol organic enrichment and the resulting impact on water uptake over the remote Southern Hemisphere are scarce, and therefore the region is under-represented in existing parameterisations. The Surface Ocean Aerosol Production (SOAP) voyage was a 23 d voyage which sampled three phytoplankton blooms in the highly productive water of the Chatham Rise, east of New Zealand. In this study we examined the enrichment of organics to nascent sea spray aerosol and the modifications to sea spray aerosol water uptake using in situ chamber measurements of seawater samples taken during the SOAP voyage.