The Sahel region of West Africa experiences decadal swings between periods of drought and abundant rainfall, and a large body of work asserts that these variations in the West African monsoon are a ...response to changes in the temperatures of the tropical Atlantic and Indian Oceans. However, here it is shown that when forced by SST alone, most state-of-the-art climate models do not reproduce a statistically significant upward trend in Sahelian precipitation over the last 30 years and that those models with a significant upward trend in rainfall seem to achieve this result for disparate reasons. Here the role of the Saharan heat low (SHL) in the recovery from the Sahelian drought of the 1980s is examined. Using observations and reanalyses, it is demonstrated that there has been an upward trend in SHL temperature that is coincident with the drought recovery. A heat and moisture budget analysis of the SHL suggests that the rise in temperature is due to greenhouse warming by water vapor, but that changes in water vapor are strongly dependent upon the temperature of the SHL: a process termed the Saharan water vapor–temperature (SWAT) feedback. It is shown that the structure of the drought recovery is consistent with a warming SHL and is evidence of a fundamental, but not exclusive, role for the SHL in the recent increase in Sahelian monsoon rainfall.
Urban aerosol microphysical and optical properties were investigated over the Paris area coupling, for the first time, with dedicated airborne in situ instruments (nephelometer and particle sizers) ...and active remote sensor (lidar) as well as ground‐based in situ instrumentation. The experiment, covering two representative pollution events, was conducted in the framework of the Etude et Simulation de la Qualité de l'air en Ile de France (ESQUIF) program. Pollution plumes were observed under local northerly and southerly synoptic wind conditions on 19 and 31 July 2000, respectively. The 19 July (31 July) event was characterized by north‐northwesterly (westerly) advection of polluted (clean) air masses originating from Great Britain (the Atlantic Ocean). The aerosol number size distribution appeared to be composed mainly of two modes in the planetary boundary layer (accumulation and nucleation) and three modes in the surface layer (accumulation, nucleation, and coarse). The characteristics of the size distribution (modal radii and geometric dispersion) were remarkably similar on both days and very coherent with the aerosol optical parameters retrieved from lidar and nephelometer measurements. The city of Paris mainly produces aerosols in the nucleation mode (modal radius of ∼0.03 μm) that have little influence on the aerosol optical properties in the visible spectral range. The latter are largely dominated by the scattering properties of aerosols in the accumulation mode (modal radius of ∼0.12 μm). When the incoming air mass is already polluted (clear), the aerosol in the accumulation mode is shown to be essentially hydrophobic (hydrophilic) in the outgoing air mass.
The radiative effects of biomass burning aerosols (BBAs) on low-level atmospheric circulation over southern Africa are investigated on 5 September 2017 during the Aerosols, Radiation and Clouds in ...southern Africa (AEROCLO-sA) field campaign. This is conducted using a variety of in situ and remote sensing observations, as well as 5-day twin ensemble simulations made with the Meso-NH mesoscale model, one including the direct and semi-direct radiative effects of aerosols and one in which these effects are not included. We show that the radiative impact of BBA building up over a period of 5 days in the Meso-NH simulations can lead to significantly different circulations at low-and mid-levels, thereby affecting dust emissions over southern Namibia and northwestern South Africa as well as the transport of BBA in a so-called "river of smoke". While most of the regional scale dynamics, thermodynamics and composition features are convincingly represented in the simulation with BBA radiative effects, neglecting the radiative impact of BBA leads to unrealistic representations of (i) the low-level jet (LLJ) over the plateau plateau, which is the main low-level dynamic feature fostering dust emission, and (ii) the mid-level dynamics pertaining to the transport of BBA from the fire-prone regions in the Tropics to the mid-latitudes. For instance, when the BBA radiative impacts are not included, the LLJ is too weak and not well established over night, and the developing convective planetary boundary layer (PBL) is too deep compared to observations. The deeper convective PBL over Etosha and surrounding areas is related to the enhanced anomalous upward motion caused by the eastern displacement of the river of smoke. This eastern displacement is, in turn, related to the weaker southerly African Easterly Jet. Both ensemble simulations provide clear evidence that the enhanced near surface extinction coefficient values detected from observations over Etosha are related to the downward mixing of BBA in the developing convective boundary layer rather that dust being emitted as a result of the LLJ breakdown after sunrise. This study suggests that the radiative effect of BBAs needs to be taken into account to properly forecast dust emissions in Namibia.
From 23 January to 13 February 2020, 20 ATR-42 scientific flights were conducted in the framework of the EUREC4A field campaign over the tropical Atlantic, off the coast of Barbados (13∘30′ N, ...-58∘30′ W). By means of a sideway-pointing lidar, these flights allowed us to retrieve the optical properties of the aerosols found in the sub-cloud layer and below the trade wind inversion. Two distinct periods with significant aerosol contents were identified in relationship with the so-called trade wind and tropical regimes, respectively. For these two regimes, mixings of two air mass types encompassing dust and carbonaceous aerosols have been highlighted. Both were mainly from West Africa with similar optical contributions and linked to dust uptake above Sahara and biomass burning between Guinea-Bissau and Côte d'Ivoire. In the tropical transport regime, the wind within the planetary boundary layer is stronger and favours a contribution of marine aerosols (sulfate and sea salt aerosol components) in shallower aerosol layers than for the trade wind transport regime. The latter is responsible for advecting dust–biomass-burning-aerosol mixtures in the deeper, well-mixed layer, in part due to the complex interactions of the easterly flow from West Africa with mid-latitude dynamics. The aerosol vertical structures appear to be well reproduced using atmospheric composition reanalyses from CAMS when comparing with lidar-derived vertical profiles. The competition between the two types of transport regimes leads to strong heterogeneity in the optical properties of the horizontal aerosol field. Our study highlights the transport regime under which a significant mixture of dust and biomass burning aerosols from West Africa can be observed over the Caribbean and Barbados in particular, namely the trade wind regime.
The Saharan heat low (SHL) plays a pivotal role in the West African monsoon system in spring and summer. The recent trend in SHL activity has been analysed using two sets of numerical weather ...prediction (NWP) model reanalyses and Atmospheric Models Intercomparison Project simulations from 15 climate models performed in the framework of the 5th Coupled Models Intercomparison Project (CMIP5) exercise. A local increase of temperature in the Sahara during the 90s is found in the two sets of NWP models temperature. This increase is stronger within the SHL region than over the surrounding areas. Using different temporal filters (under 25 days, 25–100 days and above 300 days), we show that this is accompanied by a slight but widespread increase of temperature, and a change in the filtered signal under 25 days during the transition period of the 90s. We also show that SHL pulsations occurring at different time scales impact the West Africa climate on a variety of spatial scales, from the regional scale (for the high band pass) to the synoptic scale (for the low band pass signal). Despite a large variability in the temporal trends for 15 climate models from the CMIP5 project, the warming trend in the 90s is observed in the models ensemble mean. Nevertheless, large discrepancies are found between the NWP models reanalyses and the climate model simulations regarding the spatial and temporal evolutions of the SHL as well as its impact on West African climate at the different time scales. These comparisons also reveal that climate models represent the West African monsoon interactions with SHL pulsations quite differently. We provide recommendations to use some of them depending on the time scales of the processes at play (synoptic, seasonal, interannual) and based on key SHL metrics (location, mean intensity, global trend, interaction with the West African monsoon dynamics).
In this work, we compare IASI-retrieved vertical water vapour profiles and related precipitable water over a complex region, namely the Rhine Valley area, during the pre-operational period of IASI ...exploitation (June?August 2007). Both IASI water vapour mixing ratio profiles and integrated water vapour content are retrieved from L1C radiances spectra using two techniques and compared with water vapour related observations acquired during the Convective and Orographically-induced Precipitation Study (COPS) field campaign that took place in this area at that time (i.e. lidars, radiosoundings and a global positioning system - GPS - station network). This work addresses the issue of IASI vertical spatial resolution and its capability to detect two-layer water vapour structures such as those observed in a mountainous area and which play an important role in convective initiation or inhibition. We found that this capability mostly relies on the type of a-priori background vector (climatology or space-time colocated ECMWF analysis), which is used within the retrieval scheme. Systematic comparison of water vapour products derived from 71 IASI spectra confirms that IASI can retrieve water vapour amounts in 2 km width layers, in the lower troposphere, with an accuracy of approximately 10%.
Direct and semi‐direct radiative effects of biomass burning aerosols (BBA) from southern and central African fires are still widely debated, in particular because climate models have been ...unsuccessful in reproducing the low single scattering albedo in BBA over the eastern Atlantic Ocean. Using state‐of‐the‐art airborne in situ measurements and Mie scattering simulations, we demonstrate that low single scattering albedo in well‐aged BBA plumes over southern West Africa results from the presence of strongly absorbing refractory black carbon (rBC), whereas the brown carbon contribution to the BBA absorption is negligible. Coatings enhance light absorption by rBC‐containing particles by up to 210%. Our results show that accounting for the diversity in black carbon mixing state by combining internal and external configurations is needed to accurately estimate the optical properties and henceforth the shortwave direct radiative effect and heating rate of BBA over southern West Africa.
Plain Language Summary
Extensive seasonal fires over southern and central Africa result in the transport of massive amounts of biomass burning aerosols over huge areas of the eastern Atlantic Ocean. Recent field observations highlight that biomass burning aerosols transported from the coast of southern Africa to the far north over southern West Africa were characterized by low single scattering albedo. This finding is of paramount interest, because radiative heating within the absorbing aerosol layer is hypothesized to affect the low cloud deck over this specific region and may ultimately influence the large‐scale circulation. However, debate remains about the causes of the low single scattering albedo by biomass burning aerosols, causing ambiguous parameterizations of their optical properties in climate models. Here we present simultaneous airborne measurements of the composition and optical properties of biomass burning aerosols transported over southern West Africa. We show that black carbon particles dominated the light absorption by biomass burning aerosols at mid‐visible wavelengths. Our findings indicate that the black carbon mixing state plays a significant role in the aerosol optical properties and may be an important modulator to be considered in climate models for simulating direct and semi‐direct radiative effects of biomass burning aerosol over southern West Africa.
Key Points
The low single scattering albedo in biomass burning aerosol (BBA) over southern West Africa results from the presence of refractory black carbon
The brown carbon contribution to the aerosol absorption is negligible in these well‐aged BBA plumes
Accounting for the diversity in black carbon mixing state is needed to accurately estimate BBA optical properties
The radiative effects of biomass burning aerosols (BBAs) on low-level atmospheric circulation over southern Africa are investigated on 5 September 2017 during the Aerosols, Radiation and Clouds in ...southern Africa (AEROCLO-sA) field campaign. This is conducted using a variety of in situ and remote sensing observations, as well as two 5 d ensemble simulations made with the Meso-NH mesoscale model, one including the direct and semi-direct radiative effects of aerosols and one in which these effects are not included. We show that the radiative impact of BBA building up over a period of 5 d in the Meso-NH simulations can lead to significantly different circulations at low and middle levels, thereby affecting dust emissions over southern Namibia and northwestern South Africa as well as the transport of BBA in a so-called “river of smoke”. While most of the regional-scale dynamics, thermodynamics and composition features are convincingly represented in the simulation with BBA radiative effects, neglecting the radiative impact of BBA leads to unrealistic representations of (i) the low-level jet (LLJ) over the plateau, which is the main low-level dynamic feature fostering dust emission, and (ii) the mid-level dynamics pertaining to the transport of BBA from the fire-prone regions in the tropics to the mid-latitudes. For instance, when the BBA radiative impacts are not included, the LLJ is too weak and not well established over night, and the developing convective planetary boundary layer (PBL) is too deep compared to observations. The deeper convective PBL over Etosha and surrounding areas is related to the enhanced anomalous upward motion caused by the eastern displacement of the river of smoke. This eastern displacement is, in turn, related to the weaker southerly African easterly jet. Both ensemble simulations provide clear evidence that the enhanced near-surface extinction coefficient values detected from observations over Etosha are related to the downward mixing of BBA in the developing convective boundary layer rather than dust being emitted as a result of the LLJ breakdown after sunrise. This study suggests that the radiative effect of BBAs needs to be taken into account to properly forecast dust emissions in Namibia.
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