The recently commissioned Linac Coherent Light Source is an X-ray free-electron laser at the SLAC National Accelerator Laboratory. It produces coherent soft and hard X-rays with peak brightness ...nearly ten orders of magnitude beyond conventional synchrotron sources and a range of pulse durations from 500 to <10 fs (10-15 s). With these beam characteristics this light source is capable of imaging the structure and dynamics of matter at atomic size and timescales. The facility is now operating at X-ray wavelengths from 22 to 1.2 A and is presently delivering this high-brilliance beam to a growing array of scientific researchers. We describe the operation and performance of this new 'fourth-generation light source'.
The X-ray free-electron laser has opened a new era for photon science, improving the X-ray brightness by ten orders of magnitude over previously available sources. Similar to an optical laser, the ...spectral and temporal structure of the radiation pulses can be tailored to the specific needs of many experiments by accurately manipulating the lasing medium, that is, the electron beam. Here we report the generation of mJ-level two-colour hard X-ray pulses of few femtoseconds duration with an XFEL driven by twin electron bunches at the Linac Coherent Light Source. This performance represents an improvement of over an order of magnitude in peak power over state-of-the-art two-colour XFELs. The unprecedented intensity and temporal coherence of this new two-colour X-ray free-electron laser enable an entirely new set of scientific applications, ranging from X-ray pump/X-ray probe experiments to the imaging of complex biological samples with multiple wavelength anomalous dispersion.
The Linac Coherent Light Source is a SASE x-ray free-electron laser (FEL) project presently under construction at SLAC J. Arthur et al., SLAC-R-593, 2002.. The injector section, from drive laser and ...rf photocathode gun through first bunch compressor chicane, was installed in the fall of 2006. The initial system commissioning with an electron beam was completed in August of 2007, with the goal of a 1.2-micron emittance in a 1-nC bunch demonstrated. The second phase of commissioning, including second bunch compressor and full linac, is planned for 2008, with FEL commissioning in 2009. We report experimental results and experience gained in the first phase of commissioning, including the photocathode drive laser, rf gun, photocathode, S-band and X-band rf systems, first bunch compressor, and the various beam diagnostics.
The very bright electron beam required for an x-ray free-electron laser (FEL), such as the linac coherent light source (LCLS), is susceptible to a microbunching instability in the magnetic bunch ...compressors, prior to the FEL undulator. The uncorrelated electron energy spread in the LCLS can be increased by an order of magnitude to provide strong Landau damping against the instability without degrading the FEL performance. To this end, a “laser-heater” system has been installed in the LCLS injector, which modulates the energy of a 135-MeV electron bunch with an IR-laser beam in a short undulator, enclosed within a four-dipole chicane. In this paper, we report detailed measurements of laser-heater-induced energy spread, including the unexpected self-heating phenomenon when the laser energy is very low. We discuss the suppression of the microbunching instability with the laser heater and its impact on the x-ray FEL performance. We also present the analysis of these experimental results and develop a three-dimensional longitudinal space charge model to explain the self-heating effect.
Molecular oxygen (O
2
) migration in isolated β-chains of human hemoglobin was studied using molecular dynamics simulations and laser kinetic absorption spectroscopy. Insertion of xenon (Xe) atoms ...into the isolated chains was found to decrease the time constant of the slowest component of geminal O
2
rebinding to the protein. This change was caused by a decrease in the intra-protein space available for O
2
migration after insertion of the inert gas into the Xe-binding sites of the protein. Molecular dynamics simulations revealed that the O
2
molecule occupied both the Xe2 and Xe1 sites of the protein during geminal recombination to the isolated β-chains. The amino acids involved in formation of the primary and secondary docking sites of the protein were determined. The results are important for understanding the mechanism of O
2
binding by both native tetrameric human hemoglobin and artificial oxygen carriers based on heme proteins.
For the Linac Coherent Light Source II (LCLS-II) project at SLAC, a 1.3 GHz superconducting rf (SRF) linac is being constructed that will generate 4 GeV electron bunches at a high repetition rate to ...drive x-ray free electron lasers. The LCLS-II electron source, which comprises the first three meters of the electron injector, includes two normal-conducting, continuous-wave rf cavities: a one-cell, 185.7 MHz gun and a two-cell, 1.3 GHz buncher. It also includes a gun load-lock system that allows photocathodes to be changed under vacuum. The components in this beam-line section were designed and built by Lawrence Berkeley National Laboratory based on experience from their advanced photoinjector experiment program. In combination with the SLAC UV laser system, the electron source is designed to produce beam rates up to 1 MHz with average currents up to30μAinitially. The source was installed in mid-2018, well in advance of the SRF linac, which is now nearing completion. The source was commissioned over a two-year period, and this paper presents results including electron beam and dark current characterization.