Low-cost sensors for particulate matter mass (PM) enable spatially dense, high temporal resolution measurements of air quality that traditional reference monitoring cannot. Low-cost PM sensors are ...especially beneficial in low and middle-income countries where few, if any, reference grade measurements exist and in areas where the concentration fields of air pollutants have significant spatial gradients. Unfortunately, low-cost PM sensors also come with a number of challenges that must be addressed if their data products are to be used for anything more than a qualitative characterization of air quality. The various PM sensors used in low-cost monitors are all subject to biases and calibration dependencies, corrections for which range from relatively straightforward (e.g. meteorology, age of sensor) to complex (e.g. aerosol source, composition, refractive index). The methods for correcting and calibrating these biases and dependencies that have been used in the literature likewise range from simple linear and quadratic models to complex machine learning algorithms. Here we review the needs and challenges when trying to get high-quality data from low-cost sensors. We also present a set of best practices to follow to obtain high-quality data from these low-cost sensors.
•Low-cost sensors (LCS) give air pollution data at high spatial/temporal resolution.•Challenges in obtaining high quality data from low-cost PM sensors are reviewed.•Current methods of correcting LCS data are reviewed, best practices are suggested.•To better evaluate LCS corrections, both accuracy and bias should be reported.
The unintended climatic implications of aerosol and precursor emission reductions implemented to protect public health are poorly understood. We investigate the precipitation response to regional ...changes in aerosol emissions using three coupled chemistry-climate models: NOAA Geophysical Fluid Dynamics Laboratory Coupled Model 3 (GFDL-CM3), NCAR Community Earth System Model (CESM1), and NASA Goddard Institute for Space Studies ModelE2 (GISS-E2). Our approach contrasts a long present-day control simulation from each model (up to 400 years with perpetual year 2000 or 2005 emissions) with 14 individual aerosol emissions perturbation simulations (160-240 years each). We perturb emissions of sulfur dioxide and/or carbonaceous aerosol within six world regions and assess the significance of precipitation responses relative to internal variability determined by the control simulation and across the models. Global and regional precipitation mostly increases when we reduce regional aerosol emissions in the models, with the strongest responses occurring for sulfur dioxide emissions reductions from Europe and the United States. Precipitation responses to aerosol emissions reductions are largest in the tropics and project onto the El Nino Southern Oscillation (ENSO). Regressing precipitation onto an Indo-Pacific zonal sea level pressure gradient index (a proxy for ENSO) indicates that the ENSO component of the precipitation response to regional aerosol removal can be as large as 20% of the total simulated response. Precipitation increases in the Sahel in response to aerosol reductions in remote regions because an anomalous interhemispheric temperature gradient alters the position of the Intertropical Convergence Zone (ITCZ). This mechanism holds across multiple aerosol reduction simulations and models.
The climatic implications of regional aerosol and precursor emissions reductions implemented to protect human health are poorly understood. We investigate the mean and extreme temperature response to ...regional changes in aerosol emissions using three coupled chemistry–climate models: NOAA GFDL CM3, NCAR CESM1, and NASA GISS-E2. Our approach contrasts a long present-day control simulation from each model (up to 400 years with perpetual year 2000 or 2005 emissions) with 14 individual aerosol emissions perturbation simulations (160–240 years each). We perturb emissions of sulfur dioxide (SO2) and/or carbonaceous aerosol within six world regions and assess the statistical significance of mean and extreme temperature responses relative to internal variability determined by the control simulation and across the models. In all models, the global mean surface temperature response (perturbation minus control) to SO2 and/or carbonaceous aerosol is mostly positive (warming) and statistically significant and ranges from +0.17 K (Europe SO2) to -0.06 K (US BC). The warming response to SO2 reductions is strongest in the US and Europe perturbation simulations, both globally and regionally, with Arctic warming up to 1 K due to a removal of European anthropogenic SO2 emissions alone; however, even emissions from regions remote to the Arctic, such as SO2 from India, significantly warm the Arctic by up to 0.5 K. Arctic warming is the most robust response across each model and several aerosol emissions perturbations. The temperature response in the Northern Hemisphere midlatitudes is most sensitive to emissions perturbations within that region. In the tropics, however, the temperature response to emissions perturbations is roughly the same in magnitude as emissions perturbations either within or outside of the tropics. We find that climate sensitivity to regional aerosol perturbations ranges from 0.5 to 1.0 K (W m(exp -2))(exp -1) depending on the region and aerosol composition and is larger than the climate sensitivity to a doubling of CO2 in two of three models. We update previous estimates of regional temperature potential (RTP), a metric for estimating the regional temperature responses to a regional emissions perturbation that can facilitate assessment of climate impacts with integrated assessment models without requiring computationally demanding coupled climate model simulations. These calculations indicate a robust regional response to aerosol forcing within the Northern Hemisphere midlatitudes, regardless of where the aerosol forcing is located longitudinally. We show that regional aerosol perturbations can significantly increase extreme temperatures on the regional scale. Except in the Arctic in the summer, extreme temperature responses largely mirror mean temperature responses to regional aerosol perturbations through a shift of the temperature distributions and are mostly dominated by local rather than remote aerosol forcing.
Previous studies demonstrated that global warming can lead to deteriorated air quality even when anthropogenic emissions were kept constant, which has been called a climate change penalty on air ...quality. It is expected that anthropogenic emissions will decrease significantly in the future considering the aggressive emission control actions in China. However, the dependence of climate change penalty on the choice of emission scenario is still uncertain. To fill this gap, we conducted multiple independent model simulations to investigate the response of PM2.5 to future (2050) climate warming (RCP8.5) in China but with different emission scenarios, including the constant 2015 emissions, the 2050 CLE emissions (based on Current Legislation), and the 2050 MTFR emissions (based on Maximum Technically Feasible Reduction). For each set of emissions, we estimate climate change penalty as the difference in PM2.5 between a pair of simulations with either 2015 or 2050 meteorology. Under 2015 emissions, we find a PM2.5 climate change penalty of 1.43 μg m−3 in Eastern China, leading to an additional 35,000 PM2.5-related premature deaths 95% confidence interval (CI), 21,000-40,000 by 2050. However, the PM2.5 climate change penalty weakens to 0.24 μg m−3 with strict anthropogenic emission controls under the 2050 MTFR emissions, which decreases the associated PM2.5-related deaths to 17,000. The smaller MTFR climate change penalty contributes 14% of the total PM2.5 decrease when both emissions and meteorology are changed from 2015 to 2050, and 24% of total health benefits associated with this PM2.5 decrease in Eastern China. This finding suggests that controlling anthropogenic emissions can effectively reduce the climate change penalty on PM2.5 and its associated premature deaths, even though a climate change penalty still occurs even under MTFR. Strengthened controls on anthropogenic emissions are key to attaining air quality targets and protecting human health in the context of future global climate change.
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•Future climate under RCP8.5 will increase PM2.5 by over 1 μg m−3 in Eastern China.•14% of PM2.5 decrease from emission controls occurs by reducing climate penalty.•Over one-third of PM2.5-mortality can be avoided after strict emission reductions.
Atmospheric new particle formation (NPF) is a crucial process driving aerosol number concentrations in the atmosphere; it can significantly impact the evolution of atmospheric aerosol and cloud ...processes. This study analyses at least 1 year of asynchronous particle number size distributions from six different locations in India. We also analyze the frequency of NPF and its contribution to cloud condensation nuclei (CCN) concentrations. We found that the NPF frequency has a considerable seasonal variability. At the measurement sites analyzed in this study, NPF frequently occurs in March–May (pre-monsoon, about 21 % of the days) and is the least common in October–November (post-monsoon, about 7 % of the days). Considering the NPF events in all locations, the particle formation rate (J_(SDS)) varied by more than 2 orders of magnitude (0.001–0.6 /cu.cm s) and the growth rate between the smallest detectable size and 25 nm (GR_(SDS-25 nm)) by about 3 orders of magnitude (0.2–17.2 nm/h). We found that JSDS was higher by nearly 1 order of magnitude during NPF events in urban areas than mountain sites. GRSDS did not show a systematic difference. Our results showed that NPF events could significantly modulate the shape of particle number size distributions and CCN concentrations in India. The contribution of a given NPF event to CCN concentrations was the highest in urban locations (4.3 × 10^(3) /cu.cm per event and 1.2 × 10^(3)/cu.cm per event for 50 and 100 nm, respectively) as compared to mountain background sites (2.7 × 10^(3)/cu.cm per event and 1.0 × 10^(3)/cu.cm per event, respectively). We emphasize that the physical and chemical pathways responsible for NPF and factors that control its contribution to CCN production require in situ field observations using recent advances in aerosol and its precursor gaseous measurement techniques.
Abstract
Belmont County, Ohio is heavily dominated by unconventional oil and gas development that results in high levels of ambient air pollution. Residents here chose to work with a national ...volunteer network to develop a method of participatory science to answer questions about the association between impact on the health of their community and pollution exposure from the many industrial point sources in the county and surrounding area and river valley. After first directing their questions to the government agencies responsible for permitting and protecting public health, residents noted the lack of detailed data and understanding of the impact of these industries. These residents and environmental advocates are using the resulting science to open a dialogue with the EPA in hopes to ultimately collaboratively develop air quality standards that better protect public health. Results from comparing measurements from a citizen-led participatory low-cost, high-density air pollution sensor network of 35 particulate matter and 25 volatile organic compound sensors against regulatory monitors show low correlations (consistently R
2
< 0.55). This network analysis combined with complementary models of emission plumes are revealing the inadequacy of the sparse regulatory air pollution monitoring network in the area, and opening many avenues for public health officials to further verify people’s experiences and act in the interest of residents’ health with enforcement and informed permitting practices. Further, the collaborative best practices developed by this study serve as a launchpad for other community science efforts looking to monitor local air quality in response to industrial growth.
The contribution of individual aerosol species and greenhouse gases to precipitation changes during the South Asian summer monsoon is uncertain. Mechanisms driving responses to anthropogenic forcings ...need further characterization. We use an atmosphere‐only climate model to simulate the fast response of the summer monsoon to different anthropogenic aerosol types and to anthropogenic greenhouse gases. Without normalization, sulfate is the largest driver of precipitation change between 1850 and 2000, followed by black carbon and greenhouse gases. Normalized by radiative forcing, the most effective driver is black carbon. The precipitation and moisture budget responses to combinations of aerosol species perturbed together scale as a linear superposition of their individual responses. We use both a circulation‐based and moisture budget‐based argument to identify mechanisms of aerosol and greenhouse gas induced changes to precipitation, and find that in all cases the dynamic contribution is the dominant driver to precipitation change in the monsoon region.
The unintended consequences of reductions in regional anthropogenic sulfur dioxide (SO2) emissions implemented to protect human health are poorly understood. SO2 decreases began in the 1970s in the ...US and Europe and are expected to continue into the future, while recent emissions decreases in China are also projected to continue. In addition to the well-documented climate effects (warming) from reducing aerosols, tropospheric oxidation is impacted via aerosol modification of photolysis rates and radical sinks. Impacts on the hydroxyl radical and other trace constituents directly affect climate and air quality metrics such as surface ozone levels. We use the Geophysical Fluid Dynamics Laboratory Atmospheric Model version 3 nudged towards National Centers for Environmental Prediction (NCEP) reanalysis wind velocities to estimate the impact of SO2 emissions from the US, Europe, and China by differencing a control simulation with an otherwise identical simulation in which 2015 anthropogenic SO2 emissions are set to zero over one of the regions. Springtime sulfate aerosol changes occur both locally to the emission region and also throughout the Northern Hemispheric troposphere, including remote oceanic regions and the Arctic. Hydroperoxy (HO2) radicals are directly removed via heterogeneous chemistry on aerosol surfaces, including sulfate, in the model, and we find that sulfate aerosol produced by SO2 emissions from the three individual northern mid-latitude regions strongly reduces both HO2 and hydroxyl (OH) by up to 10 % year-round throughout most of the troposphere north of 30∘ N latitude. Regional SO2 emissions significantly increase nitrogen oxides (NOx) by about 5 %–8 % throughout most of the free troposphere in the Northern Hemisphere by increasing the NOx lifetime as the heterogeneous sink of HO2 on sulfate aerosol declines. Despite the NOx increases, tropospheric ozone decreases at northern mid-latitudes by 1 %–4 % zonally averaged and by up to 5 ppbv in summertime surface air over China, where the decreases in HO2 and OH suppress O3 production. Since 2015 anthropogenic SO2 emissions in China exceed those in the US or Europe, the oxidative response is greatest for the China perturbation simulation. Chemical effects of aerosols on oxidation (reactive uptake) dominate over radiative effects (photolysis rates), the latter of which are only statistically significant locally for the large perturbation over China. We find that the SO2 emissions decrease in China, which has yet to be fully realized, will have the largest impact on oxidants and related species in the Northern Hemisphere free troposphere compared to future decreases in Europe or the US. Our results bolster previous calls for a multipollutant strategy for air pollution mitigation to avoid the unintended consequence of aerosol removal leading to surface ozone increases that offset or mask surface ozone gains achieved by regulation of other pollutants, especially in countries where current usage of high-sulfur emitting fuels may be phased out in the future.
Dry deposition (DD) is a major loss process for tropospheric ozone and some reactive nitrogen and carbon precursors. We investigate the response of summertime ozone and its production chemistry over ...the Southeast United States (USA) to variability in this sink. Turning off DD of oxidized nitrogen, ozone, or all species over the United States in the Geophysical Fluid Dynamics Laboratory AM3 model increases regional mean surface ozone by 5, 18, or 25 ppb, respectively. Additional sensitivity simulations demonstrate that, assuming linearity, surface ozone has a similar sensitivity to ozone DD as to NOx emissions. Trends in ozone production efficiency derived from observed relationships between ozone and precursor oxidation products may not solely reflect precursor emission changes if ozone DD varies (e.g., with meteorology). We conclude that DD variability merits consideration when interpreting observed ozone trends. Quantifying the impact of changes in sinks versus sources will require long‐term DD measurements across the region of interest.
Climate models suggest that anthropogenic aerosol‐induced drying dominates the historical rainfall changes over the heavily populated South Asian monsoon region. The regional response depends on both ...the aerosol fast radiative effect and the slow process through sea surface temperature (SST) cooling. Two atmospheric general circulation models, NCAR‐CAM5 and GFDL‐AM3, are used to investigate the monsoon response to prescribed aerosol‐forced SSTs. The total SST is separated into uniform cooling and a spatially varying component characterized by interhemispheric asymmetry. The monsoon rainfall is predominantly controlled by the nonuniform SSTs, in the local Indian Ocean, South, and East China Seas (IO‐CSs). The reduced meridional SST gradient in the IO‐CSs leads to weakened monsoon circulation, which drives a north‐south dipole rainfall change. The latitudinal location of the dipole shows model dependence due to differences in local SSTs and their meridional gradient, which determines the latitudinal location of the meridional overturning circulation responses.
Plain Language Summary
South Asian monsoon rainfall is an important part of the region's economy as it affects the agriculture and water supply in this densely populated region. Anomalously weak monsoon rainfall can lead to catastrophic crop failures and famine. Recent increases in aerosol emission not only caused severe air pollution problems in the region, but also led to monsoon circulation and rainfall changes. Previous studies have shown that aerosols can lead to drying in a region due to interaction with radiation and clouds. Additionally, the northern hemisphere centric aerosol emission led sea surface temperatures to cool more in northern than southern hemispheres. This sea surface temperature mediated responses to aerosol can play an important role in the South Asian monsoon response to aerosols. In this study, we demonstrate that this effect is mainly through the north‐south temperature gradient in the Indian Ocean, South, and East China Seas, which leads to atmospheric circulation that weakens the monsoon overturning and drying in South Asia. However, the exact latitudes of this drying tend to be highly model‐dependent due to different sea surface temperatures in the local ocean basins.
Key Points
Predominant impact of aerosol‐forced sea surface temperatures on South Asian monsoon is the local spatially nonuniform part
Large intermodel differences in monsoon responses are due to regional aerosol‐forced SST differences
Dynamical mechanisms dominate South Asian drying due to SST‐mediated aerosol forcing
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