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Jiang, Bing; Zhao, Meng; Li, Shu‐Sen; Xu, Yun‐He; Loh, Teck‐Peng
Angewandte Chemie International Edition, January 8, 2018, Letnik: 57, Številka: 2Journal Article
A RhIII‐catalyzed intramolecular oxidative cross‐coupling between double bonds for the synthesis of macrolides is described. Under the optimized reaction conditions, macrocycles containing a diene moiety can be formed in reasonable yields and with excellent chemo‐ and stereoselectivity. This method provides an efficient approach to synthesize macrocyclic compounds containing a 1,3‐conjugated diene structure. Two pair: A RhIII‐catalyzed intramolecular oxidative cross‐coupling between double bonds for the synthesis of macrolides is described. Under the optimized conditions, macrocycles containing a diene moiety can be formed in reasonable yields and with excellent chemo‐ and stereoselectivity. This provides efficient access to macrocyclic compounds containing 1,3‐conjugated dienes.
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