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Li, Pengsong; Wang, Maoyu; Duan, Xinxuan; Zheng, Lirong; Cheng, Xiaopeng; Zhang, Yuefei; Kuang, Yun; Li, Yaping; Ma, Qing; Feng, Zhenxing; Liu, Wen; Sun, Xiaoming
Nature communications, 04/2019, Letnik: 10, Številka: 1Journal Article
Single atom catalyst, which contains isolated metal atoms singly dispersed on supports, has great potential for achieving high activity and selectivity in hetero-catalysis and electrocatalysis. However, the activity and stability of single atoms and their interaction with support still remains a mystery. Here we show a stable single atomic ruthenium catalyst anchoring on the surface of cobalt iron layered double hydroxides, which possesses a strong electronic coupling between ruthenium and layered double hydroxides. With 0.45 wt.% ruthenium loading, the catalyst exhibits outstanding activity with overpotential 198 mV at the current density of 10 mA cm and a small Tafel slope of 39 mV dec for oxygen evolution reaction. By using operando X-ray absorption spectroscopy, it is disclosed that the isolated single atom ruthenium was kept under the oxidation states of 4+ even at high overpotential due to synergetic electron coupling, which endow exceptional electrocatalytic activity and stability simultaneously.
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JCR | SNIP | JCR | SNIP | JCR | SNIP | JCR | SNIP |
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