When two atomic layers are brought into contact at a relative twist angle, a large-scale pattern, called a moiré superlattice, emerges due to the (angular or lattice) mismatch between the layers. ...This has profound consequences in terms of the Hamiltonian of the system but was also considered in several publications as a means to extract the local strain tensor. While extracting the twist angle based on knowledge of the periodicity of the moiré is trivial in the case of a regular moiré pattern, in many examples in the literature, that is not the case. In particular, extracting the strain tensor and twist angle maps from a spatially varying moiré pattern is not straightforward. This article aims to provide a practical tool to extract the strain tensor and twist angle from an experimentally observable pattern. It further addresses the limitation of any such approach in the absence of additional experimental information beyond the moiré superlattice pattern.
We report a combined nano-photocurrent and infrared nanoscopy study of twisted bilayer graphene (TBG) enabling access to the local electronic phenomena at length scales as short as 20 nm. We show ...that the photocurrent changes sign at carrier densities tracking the local superlattice density of states of TBG. We use this property to identify domains of varying local twist angle by local photothermoelectric effect. Consistent with the photocurrent study, infrared nanoimaging experiments reveal optical conductivity features dominated by twist-angle-dependent interband transitions. Our results provide a fast and robust method for mapping the electronic structure of TBG and suggest that similar methods can be broadly applied to probe electronic inhomogeneities of Moiré superlattices in other van der Waals heterostructures.
A remarkable manifestation of the quantum character of electrons in matter is offered by graphene, a single atomic layer of graphite. Unlike conventional solids where electrons are described with the ...Schrödinger equation, electronic excitations in graphene are governed by the Dirac hamiltonian. Some of the intriguing electronic properties of graphene, such as massless Dirac quasiparticles with linear energy-momentum dispersion, have been confirmed by recent observations. Here, we report an infrared spectromicroscopy study of charge dynamics in graphene integrated in gated devices. Our measurements verify the expected characteristics of graphene and, owing to the previously unattainable accuracy of infrared experiments, also uncover significant departures of the quasiparticle dynamics from predictions made for Dirac fermions in idealized, free-standing graphene. Several observations reported here indicate the relevance of many-body interactions to the electromagnetic response of graphene.
Abstract
Polaritons in hyperbolic van der Waals materials—where principal axes have permittivities of opposite signs—are light-matter modes with unique properties and promising applications. ...Isofrequency contours of hyperbolic polaritons may undergo topological transitions from open hyperbolas to closed ellipse-like curves, prompting an abrupt change in physical properties. Electronically-tunable topological transitions are especially desirable for future integrated technologies but have yet to be demonstrated. In this work, we present a doping-induced topological transition effected by plasmon-phonon hybridization in graphene/α-MoO
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heterostructures. Scanning near-field optical microscopy was used to image hybrid polaritons in graphene/α-MoO
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. We demonstrate the topological transition and characterize hybrid modes, which can be tuned from surface waves to bulk waveguide modes, traversing an exceptional point arising from the anisotropic plasmon-phonon coupling. Graphene/α-MoO
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heterostructures offer the possibility to explore dynamical topological transitions and directional coupling that could inspire new nanophotonic and quantum devices.
We use low energy optical spectroscopy and first principles local density approximation plus dynamical mean field theory calculations to test the hypothesis that the anomalous transport properties of ...strongly correlated metals originate in the strong temperature dependence of their underlying resilient quasiparticles. We express the resistivity in terms of an effective plasma frequency ω(p)* and an effective scattering rate 1/τ(tr)*. We show that in the archetypal correlated material V₂O₃, ω(p)* increases with increasing temperature, while the plasma frequency from the partial sum rule exhibits the opposite trend. 1/τ(tr)* has a more pronounced temperature dependence than the scattering rate obtained from the extended Drude analysis. The theoretical calculations of these quantities are in quantitative agreement with experiment. We conjecture that these are robust properties of all strongly correlated metals, and test the conjecture by carrying out a similar analysis on thin film NdNiO₃ on a LaAlO₃ substrate.
Quantum materials are amenable to nonequilibrium manipulation with light, enabling modification and control of macroscopic properties. Light-based augmentation of superconductivity is particularly ...intriguing. Copper-oxide superconductors exhibit complex interplay between spin order, charge order, and superconductivity, offering the prospect of enhanced coherence by altering the balance between competing orders. We utilize terahertz time-domain spectroscopy to monitor the c-axis Josephson plasma resonance (JPR) in La2−xBaxCuO4 (x = 0.115) as a direct probe of superconductivity dynamics following excitation with near-infrared pulses. Starting from the superconducting state, c-axis polarized excitation with a fluence of 100 μJ/cm2 results in an increase of the far-infrared spectral weight by more than an order of magnitude as evidenced by a blueshift of the JPR, interpreted as resulting from nonthermal collapse of the charge order. The photoinduced signal persists well beyond our measurement window of 300 ps and exhibits signatures of spatial inhomogeneity. The electrodynamic response of this metastable state is consistent with enhanced superconducting fluctuations. Our results reveal that La2−xBaxCuO4 is highly sensitive to nonequilibrium excitation over a wide fluence range, providing an unambiguous example of photoinduced modification of order-parameter competition.
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