A
bstract
Neutrinoless double-beta decay is a key process in particle physics. Its experimental investigation is the only viable method that can establish the Majorana nature of neutrinos, providing ...at the same time a sensitive inclusive test of lepton number violation. CROSS (Cryogenic Rare-event Observatory with Surface Sensitivity) aims at developing and testing a new bolometric technology to be applied to future large-scale experiments searching for neutrinoless double-beta decay of the promising nuclei
100
Mo and
130
Te. The limiting factor in large-scale bolometric searches for this rare process is the background induced by surface radioactive contamination, as shown by the results of the CUORE experiment. The basic concept of CROSS consists of rejecting this challenging background component by pulse-shape discrimination, assisted by a proper coating of the faces of the crystal containing the isotope of interest and serving as energy absorber of the bolometric detector. In this paper, we demonstrate that ultra-pure superconductive Al films deposited on the crystal surfaces act successfully as pulse-shape modifiers, both with fast and slow phonon sensors. Rejection factors higher than 99.9% of
α
surface radioactivity have been demonstrated in a series of prototypes based on crystals of Li
2
MoO
4
and TeO
2
. We have also shown that point-like energy depositions can be identified up to a distance of
∼
1 mm from the coated surface. The present program envisions an intermediate experiment to be installed underground in the Canfranc laboratory (Spain) in a CROSS-dedicated facility. This experiment, comprising
∼
3
×
10
25
nuclei of
100
Mo, will be a general test of the CROSS technology as well as a worldwide competitive search for neutrinoless double-beta decay, with sensitivity to the effective Majorana mass down to 70 meV in the most favorable conditions.
A new R&D on lithium molybdate scintillators has begun within a project CLYMENE (Czochralski growth of Li2MoO4 crYstals for the scintillating boloMeters used in the rare EveNts sEarches). One of the ...main goals of the CLYMENE is a realization of a Li2MoO4 crystal growth line to be complementary to the one recently developed by LUMINEU in view of a mass production capacity for CUPID, a next-generation tonne-scale bolometric experiment to search for neutrinoless double-beta decay. In the present paper we report the investigation of performance and radiopurity of 158-g and 13.5-g scintillating bolometers based on a first large-mass (230 g) Li2MoO4 crystal scintillator developed within the CLYMENE project. In particular, a good energy resolution (2–7 keV FWHM in the energy range of 0.2–5 MeV), one of the highest light yield (0.97 keV/MeV) amongst Li2MoO4 scintillating bolometers, an efficient alpha particles discrimination (10σ) and potentially low internal radioactive contamination (below 0.2–0.3 mBq/kg of U/Th, but 1.4 mBq/kg of 210Po) demonstrate prospects of the CLYMENE in the development of high quality and radiopure Li2MoO4 scintillators for CUPID.
Random coincidences of events could be one of the main sources of background in the search for neutrino-less double-beta decay of
100
Mo with macro-bolometers, due to their modest time resolution. ...Scintillating bolometers as those based on Li
2
MoO
4
crystals and employed in the CROSS and CUPID experiments can eventually exploit the coincident fast signal detected in a light detector to reduce this background. However, the scintillation provides a modest signal-to-noise ratio, making difficult a pile-up pulse-shape recognition and rejection at timescales shorter than a few ms. Neganov–Trofimov–Luke assisted light detectors (NTL-LDs) offer the possibility to effectively increase the signal-to-noise ratio, preserving a fast time-response, and enhance the capability of pile-up rejection via pulse shape analysis. In this article we present: (a) an experimental work performed with a Li
2
MoO
4
scintillating bolometer, studied in the framework of the CROSS experiment, and utilizing a NTL-LD; (b) a simulation method to reproduce, synthetically, randomly coincident two-neutrino double-beta decay events; (c) a new analysis method based on a pulse-shape discrimination algorithm capable of providing high pile-up rejection efficiencies. We finally show how the NTL-LDs offer a balanced solution between performance and complexity to reach background index
∼
10
-
4
counts/keV/kg/year with 280 g Li
2
MoO
4
(
100
Mo enriched) bolometers at 3034 keV, the Q
β
β
of the double-beta decay, and target the goal of a next generation experiment like CUPID.
Results from a prototype TES detector for the Ricochet experiment Augier, C.; Baulieu, G.; Belov, V. ...
Nuclear instruments & methods in physics research. Section A, Accelerators, spectrometers, detectors and associated equipment,
12/2023, Volume:
1057
Journal Article
Peer reviewed
Open access
Coherent elastic neutrino-nucleus scattering (CEνNS) offers valuable sensitivity to physics beyond the Standard Model. The Ricochet experiment will use cryogenic solid-state detectors to perform a ...precision measurement of the CEνNS spectrum induced by the high neutrino flux from the Institut Laue-Langevin nuclear reactor. The experiment will employ an array of detectors, each with a mass of ∼30 g and a targeted energy threshold of 50 eV. Nine of these detectors (the “Q-Array”) will be based on a novel Transition-Edge Sensor (TES) readout style, in which the TES devices are thermally coupled to the absorber using a gold wire bond. We present initial characterization of a Q-Array-style detector using a 1 gram silicon absorber, obtaining a baseline root-mean-square resolution of less than 40 eV.
•820 g LMO crystal grown by the Czochralski method.•LMO elastic properties and stress anisotropies evaluated.•Concave tail shape generates more stresses than convex ones.
A new technology for the ...mass production of lithium molybdate (Li2MoO4) crystals needed for the realization of the cryogenic neutrinoless double-beta decay detectors is under development within the framework of the CLYMENE project. Crystals with 4 and 5 cm in diameter were grown in two different Czochralski configurations. The first configuration, based on inductive heating of a RF coil coupled with a platinum crucible, was used to grow crystals of 4 cm in diameter. Bolometric tests performed with two samples cut from a 230 g crystal have shown less performances of the large sample (158 g), which had a cleavage, as compared to the small non-cracked sample (13.5 g). Numerical modeling was applied to investigate the temperature field in the furnace, the melt convection and thermo-elastic stresses in the crystal. Numerical results reveal 30% higher thermal stress at the bottom part of the ingot in the case of a concave shape of the crystal tail (experimental case) as compared to the case of a convex shaped tail. This could explain why the fracture started at the bottom part of the 230 g crystal boule, and highlights the importance of the crystal shape in the last stage of growth process. The furnace configuration used to grow 5 cm-diameter crystals was numerically optimized in order to reduce the thermal stress in the crystals. The first kg-mass Li2MoO4 ingot grown in the optimized configuration exhibit regular shape and good structural quality.
We present the performances of two 92% enriched 130TeO2 crystals operated as thermal bolometers in view of a next generation experiment to search for neutrinoless double beta decay of 130Te. The ...crystals, 435 g each, show an energy resolution, evaluated at the 2615 keV γ-line of 208Tl, of 6.5 and 4.3 keV FWHM. The only observable internal radioactive contamination arises from 238U (15 and 8 μBq/kg, respectively). The internal activity of the most problematic nuclei for neutrinoless double beta decay, 226Ra and 228Th, are both evaluated as <3.1 μBq/kg for one crystal and <2.3 μBq/kg for the second. Thanks to the readout of the weak Cherenkov light emitted by β/γ particles by means of Neganov–Luke bolometric light detectors we were able to perform an event-by-event identification of β/γ events with a 95% acceptance level, while establishing a rejection factor of 98.21% and 99.99% for α particles.
Random coincidences of nuclear events can be one of the main background sources in low-temperature calorimetric experiments looking for neutrinoless double-beta decay, especially in those searches ...based on scintillating bolometers embedding the promising double-beta candidate
100
Mo, because of the relatively short half-life of the two-neutrino double-beta decay of this nucleus. We show in this work that randomly coinciding events of the two-neutrino double-beta decay of
100
Mo in enriched Li
2
100
MoO
4
detectors can be effectively discriminated by pulse-shape analysis in the light channel if the scintillating bolometer is provided with a Neganov–Luke light detector, which can improve the signal-to-noise ratio by a large factor, assumed here at the level of
∼
750
on the basis of preliminary experimental results obtained with these devices. The achieved pile-up rejection efficiency results in a very low contribution, of the order of
∼
6
×
10
-
5
counts/(keV
·
kg
·
y), to the background counting rate in the region of interest for a large volume (
∼
90
cm
3
) Li
2
100
MoO
4
detector. This background level is very encouraging in view of a possible use of the Li
2
100
MoO
4
solution for a bolometric tonne-scale next-generation experiment as that proposed in the CUPID project.
Growth and characterization of a Li2Mg2(MoO4)3 scintillating bolometer Danevich, F.A.; Degoda, V.Ya; Dulger, L.L. ...
Nuclear instruments & methods in physics research. Section A, Accelerators, spectrometers, detectors and associated equipment,
05/2018, Volume:
889
Journal Article
Peer reviewed
Lithium magnesium molybdate (Li2Mg2(MoO4)3) crystals were grown by the low-thermal-gradient Czochralski method. Luminescence properties of the material (emission spectra, thermally stimulated ...luminescence, dependence of intensity on temperature, phosphorescence) have been studied under X-ray excitation in the temperature interval from 8 to 400 K, while at the same being operated as a scintillating bolometer at 20 mK for the first time. We demonstrated that Li2Mg2(MoO4)3 crystals are a potentially promising detector material to search for neutrinoless double beta decay of 100Mo.
For the first time, a cadmium tungstate crystal scintillator enriched in$^{116}$ Cd has been succesfully tested as a scintillating bolometer. The measurement was performed above ground at a ...temperature of 18 mK. The crystal mass was 34.5 g and the enrichment level $\sim $ 82 %. Despite a substantial pile-up effect due to above-ground operation, the detector demonstrated high energy resolution (2–7 keV FWHM in 0.2–2.6 MeV $\gamma $ energy range and 7.5 keV FWHM at the$^{116}$ Cd double-beta decay transition energy of 2813 keV), a powerful particle identification capability and a high level of internal radio-purity. These results prove that cadmium tungstate is a promising detector material for a next-generation neutrinoless double-beta decay bolometric experiment, like that proposed in the CUPID project (CUORE Upgrade with Particle IDentification).
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