Highly Selective Solar-Driven Methanol from CO2 by a Photocatalyst/Biocatalyst Integrated System

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Highly Selective Solar-Driven Methanol from CO2 by a Photocatalyst/Biocatalyst Integrated System

Yadav, Rajesh K; Oh, Gyu Hwan; Park, No-Joong; Kumar, Abhishek; Kong, Ki-jeong; Baeg, Jin-Ook

Journal of the American Chemical Society, 12/2014, Volume: 136, Issue: 48

Journal Article

The successful development of a photocatalyst/biocatalyst integrated system that carries out selective methanol production from CO2 is reported herein. The fine-tuned system was derived from a judicious combination of graphene-based visible light active photocatalyst (CCG-IP) and sequentially coupled enzymes. The covalent attachment of isatin-porphyrin (IP) chromophore to chemically converted graphene (CCG) afforded newly developed CCG-IP photocatalyst for this research endeavor. The current work represents a new benchmark for carrying out highly selective methanol formation from CO2 in an environmentally benign manner.

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