Self-Assembly versus Directed Assembly of Nanoparticles via Pulsed Laser Induced Dewetting of Patterned Metal Films

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Self-Assembly versus Directed Assembly of Nanoparticles via Pulsed Laser Induced Dewetting of Patterned Metal Films

Fowlkes, Jason D; Kondic, Lou; Diez, Javier; Wu, Yueying; Rack, Philip D

Nano letters, 06/2011, Volume: 11, Issue: 6

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A nanoscale, synthetic perturbation was all that was required to nudge a natural, self-assembly process toward significantly higher order. Metallic thin film strips were transformed into nanoparticle arrays by nanosecond, liquid-phase dewetting. Arrays formed according to an evolving Rayleigh–Plateau instability, yet nanoparticle diameter and pitch were poorly controlled. However, by patterning a nanoscale sinusoid onto the original strip edge, a precise nanoparticle diameter and pitch emerged superseding the naturally evolving Rayleigh–Plateau instability.

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Fowlkes, Jason D | Kondic, Lou | Diez, Javier | Wu, Yueying | Rack, Philip D

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