Reaction-Driven Surface Restructuring and Selectivity Control in Allylic Alcohol Catalytic Aerobic Oxidation over Pd

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Reaction-Driven Surface Restructuring and Selectivity Control in Allylic Alcohol Catalytic Aerobic Oxidation over Pd

Lee, Adam F; Ellis, Christine V; Naughton, James N; Newton, Mark A; Parlett, Christopher M. A; Wilson, Karen

Journal of the American Chemical Society, 04/2011, Volume: 133, Issue: 15

Journal Article

Synchronous, time-resolved DRIFTS/MS/XAS cycling studies of the vapor-phase selective aerobic oxidation of crotyl alcohol over nanoparticulate Pd have revealed surface oxide as the desired catalytically active phase, with dynamic, reaction-induced Pd redox processes controlling selective versus combustion pathways.

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