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Chen, Z; Higley, D J; Beye, M; Hantschmann, M; Mehta, V; Hellwig, O; Mitra, A; Bonetti, S; Bucher, M; Carron, S; Chase, T; Jal, E; Kukreja, R; Liu, T; Reid, A H; Dakovski, G L; Föhlisch, A; Schlotter, W F; Dürr, H A; Stöhr, J
Physical review letters, 09/2018, Volume: 121, Issue: 13Journal Article
Using ultrafast ≃2.5 fs and ≃25 fs self-amplified spontaneous emission pulses of increasing intensity and a novel experimental scheme, we report the concurrent increase of stimulated emission in the forward direction and loss of out-of-beam diffraction contrast for a Co/Pd multilayer sample. The experimental results are quantitatively accounted for by a statistical description of the pulses in conjunction with the optical Bloch equations. The dependence of the stimulated sample response on the incident intensity, coherence time, and energy jitter of the employed pulses reveals the importance of increased control of x-ray free electron laser radiation.
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