The SABRE project and the SABRE Proof-of-Principle Antonello, M.; Barberio, E.; Baroncelli, T. ...
The European physical journal. C, Particles and fields,
04/2019, Letnik:
79, Številka:
4
Journal Article
Recenzirano
Odprti dostop
SABRE aims to directly measure the annual modulation of the dark matter interaction rate with NaI(Tl) crystals. A modulation compatible with the standard hypothesis, in which our Galaxy is immersed ...in a dark matter halo, has been measured by the DAMA experiment in the same target material. Other direct detection experiments, using different target materials, seem to exclude the interpretation of such modulation in the simplest scenario of WIMP-nucleon elastic scattering. The SABRE experiment aims to carry out an independent search with sufficient sensitivity to confirm or refute the DAMA claim. The goal of the SABRE experiment is to achieve the lowest background rate for a NaI(Tl) experiment (order of 0.1 cpd/kg/keV
ee
in the energy region of interest for dark matter). This challenging goal could be achievable by operating high-purity crystals inside a liquid scintillator veto for active background rejection. In addition, twin detectors will be located in the northern and southern hemispheres to identify possible contributions to the modulation from seasonal or site-related effects. The SABRE project includes an initial Proof-of-Principle phase at LNGS (Italy), to assess the radio-purity of the crystals and the efficiency of the liquid scintillator veto. This paper describes the general concept of SABRE and the expected sensitivity to WIMP annual modulation.
We present here a characterization of the low background NaI(Tl) crystal NaI-33 based on a period of almost one year of data taking (891 kg
×
days exposure) in a detector configuration with no use of ...organic scintillator veto. This remarkably radio-pure crystal already showed a low background in the SABRE Proof-of-Principle (PoP) detector, in the low energy region of interest (1–6 keV) for the search of dark matter interaction via the annual modulation signature. As the vetoable background components, such as
40
K, are here sub-dominant, we reassembled the PoP setup with a fully passive shielding. We upgraded the selection of events based on a Boosted Decision Tree algorithm that rejects most of the PMT-induced noise while retaining scintillation signals with > 90% efficiency in 1–6 keV. We find an average background of 1.39 ± 0.02 counts/day/kg/keV in the region of interest and a spectrum consistent with data previously acquired in the PoP setup, where the external veto background suppression was in place. Our background model indicates that the dominant background component is due to decays of
210
Pb, only partly residing in the crystal itself. The other location of
210
Pb is the reflector foil that wraps the crystal. We now proceed to design the experimental setup for the physics phase of the SABRE North detector, based on an array of similar crystals, using a low radioactivity PTFE reflector and further improving the passive shielding strategy, in compliance with the new safety and environmental requirements of Laboratori Nazionali del Gran Sasso.
We present new results on the radiopurity of a 3.4-kg NaI(Tl) crystal scintillator operated in the SABRE proof-of-principle detector setup. The amount of potassium contamination, determined by the ...direct counting of radioactive 40K, is found to be 2.2 ± 1.5 ppb , lowest ever achieved for NaI(Tl) crystals. With the active veto, the average background rate in the crystal in the 1–6 keV energy region of interest (ROI) is 1.20 ± 0.05 counts / day / kg / keV , which is a breakthrough since the DAMA/LIBRA experiment. Our background model indicates that the rate is dominated by 210Pb and that about half of this contamination is located in the polytetrafluoroethylene reflector. We discuss ongoing developments of the crystal manufacture aimed at the further reduction of the background, including data from purification by zone refining. A projected background rate lower than ∼ 0.2 counts / day / kg / keV in the ROI is within reach. These results represent a benchmark for the development of next-generation NaI(Tl) detector arrays for the direct detection of dark matter particles.
Ultra-pure NaI(Tl) crystals are the key element for a model-independent verification of the long standing DAMA result and a powerful means to search for the annual modulation signature of dark matter ...interactions. The SABRE collaboration has been developing cutting-edge techniques for the reduction of intrinsic backgrounds over several years. In this paper we report the first characterization of a 3.4 kg crystal, named NaI-33, performed in an underground passive shielding setup at LNGS. NaI-33 has a record low
39
K contamination of 4.3 ± 0.2 ppb as determined by mass spectrometry. We measured a light yield of 11.1 ± 0.2 photoelectrons/keV and an energy resolution of 13.2% (FWHM/E) at 59.5 keV. We evaluated the activities of
226
Ra and
228
Th inside the crystal to be
5.9
±
0.6
μ
Bq/kg and
1.6
±
0.3
μ
Bq/kg, respectively, which would indicate a contamination from
238
U and
232
Th at part-per-trillion level. We measured an activity of 0.51 ± 0.02 mBq/kg due to
210
Pb out of equilibrium and a
α
quenching factor of 0.63 ± 0.01 at 5304 keV. We illustrate the analyses techniques developed to reject electronic noise in the lower part of the energy spectrum. A cut-based strategy and a multivariate approach indicated a rate, attributed to the intrinsic radioactivity of the crystal, of
∼
1 count/day/kg/keV in the 5–20 keV region.
A series of new 1,3‐disiloxanediols has been synthesized, including naphthyl‐substituted and unsymmetrical siloxanes, and demonstrated as a new class of anion‐binding catalysts. In the absence of ...anions, diffusion‐ordered spectroscopy (DOSY) displays self‐association of 1,3‐disiloxanediols through hydrogen‐bonding interactions. Binding constants determined for 1,3‐disiloxanediol catalysts indicate strong hydrogen‐bonding and anion‐binding abilities with unsymmetrical siloxanes displaying different hydrogen‐bonding abilities for each silanol group.
Anion activation: Disiloxanediols are demonstrated as a new class of anion‐binding catalysts with NMR investigations into hydrogen bonding, self‐association, and anion‐binding constants.
The catalytic activity, kinetics, and quantification of H‐bonding ability of incompletely condensed polyhedral oligomeric silsesquioxane (POSS) silanols are reported. POSS‐triols, a homogeneous model ...for vicinal silica surface sites, exhibit enhanced H‐bonding compared with other silanols and alcohols as quantified using a 31P NMR probe. Evaluation of a Friedel–Crafts addition reaction shows that phenyl‐POSS‐triol is active as an H‐bond donor catalyst whereas other POSS silanols studied are not. An in‐depth kinetic study (using RPKA and VTNA) highlights the concentration‐dependent H‐bonding behavior of POSS‐triols, which is attributed to intermolecular association forming an off‐cycle dimeric species. Binding constants provide additional support for reduced H‐bond ability at higher concentrations, which is attributed to competitive association. POSS‐triol self‐association disrupts H‐bond donor abilities relevant for catalysis by reducing the concentration of active monomeric catalyst.
Elucidating the POSSible activity: The catalytic activity, kinetics, and quantification of H‐bonding ability of incompletely condensed polyhedral oligomeric silsesquioxane (POSS) silanols are reported. Evaluation of a Friedel–Crafts addition reaction shows that phenyl‐POSS‐triol is active as an H‐bond donor catalyst whereas other POSS silanols studied are not. Kinetic studies were carried out to highlight the concentration‐dependent H‐bonding behavior of POSS‐triols.
A prototype for a sampling calorimeter made out of cerium fluoride crystals interleaved with tungsten plates, and read out by wavelength-shifting fibres, has been exposed to beams of electrons with ...energies between 20 and 150GeV, produced by the CERN Super Proton Synchrotron accelerator complex. The performance of the prototype is presented and compared to that of a Geant4 simulation of the apparatus. Particular emphasis is given to the response uniformity across the channel front face, and to the prototype׳s energy resolution.
Growth of pure and doped TeO2 crystals for scintillating bolometers Dafinei, I.; Diemoz, M.; Longo, E. ...
Nuclear instruments & methods in physics research. Section A, Accelerators, spectrometers, detectors and associated equipment,
12/2005, Letnik:
554, Številka:
1-3
Journal Article
The High-Luminosity phase of the Large Hadron Collider at CERN (HL-LHC) poses stringent requirements on calorimeter performance in terms of resolution, pileup resilience and radiation hardness. A ...tungsten-CeF 3 sampling calorimeter is a possible option for the upgrade of current detectors. A prototype, read out with different types of wavelength-shifting fibers, has been built and exposed to high energy electrons, representative for the particle energy spectrum at HL-LHC, at the CERN SPS H4 beam line. This paper shows the performance of the prototype, mainly focussing on energy resolution and uniformity. A detailed simulation has been also developed in order to compare with data and to extrapolate to different configurations to be tested in future beam tests. Additional studies on the calorimeter and the R&D projects ongoing on the various components of the experimental setup will be also discussed.
PDF
