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Lin, J Q; Villar Arribi, P; Fabbris, G; Botana, A S; Meyers, D; Miao, H; Shen, Y; Mazzone, D G; Feng, J; Chiuzbăian, S G; Nag, A; Walters, A C; García-Fernández, M; Zhou, Ke-Jin; Pelliciari, J; Jarrige, I; Freeland, J W; Zhang, Junjie; Mitchell, J F; Bisogni, V; Liu, X; Norman, M R; Dean, M P M
Physical review letters, 2021-Feb-26, Letnik: 126, Številka: 8Journal Article
The discovery of superconductivity in a d^{9-δ} nickelate has inspired disparate theoretical perspectives regarding the essential physics of this class of materials. A key issue is the magnitude of the magnetic superexchange, which relates to whether cuprate-like high-temperature nickelate superconductivity could be realized. We address this question using Ni L-edge and O K-edge spectroscopy of the reduced d^{9-1/3} trilayer nickelates R_{4}Ni_{3}O_{8} (where R=La, Pr) and associated theoretical modeling. A magnon energy scale of ∼80 meV resulting from a nearest-neighbor magnetic exchange of J=69(4) meV is observed, proving that d^{9-δ} nickelates can host a large superexchange. This value, along with that of the Ni-O hybridization estimated from our O K-edge data, implies that trilayer nickelates represent an intermediate case between the infinite-layer nickelates and the cuprates. Layered nickelates thus provide a route to testing the relevance of superexchange to nickelate superconductivity.
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JCR | SNIP | JCR | SNIP | JCR | SNIP | JCR | SNIP |
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in: SICRIS
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