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Wang, Meng; Sui, Xuelei; Wang, Yujia; Juan, Yung-Hsiang; Lyu, Yingjie; Peng, Huining; Huang, Tongtong; Shen, Shengchun; Guo, Chenguang; Zhang, Jianbing; Li, Zhuolu; Li, Hao-Bo; Lu, Nianpeng; N'Diaye, Alpha T; Arenholz, Elke; Zhou, Shuyun; He, Qing; Chu, Ying-Hao; Duan, Wenhui; Yu, Pu
Advanced materials (Weinheim) 31, Številka: 16Journal Article
Ionic-liquid-gating- (ILG-) induced proton evolution has emerged as a novel strategy to realize electron doping and manipulate the electronic and magnetic ground states in complex oxides. While the study of a wide range of systems (e.g., SrCoO , VO , WO , etc.) has demonstrated important opportunities to incorporate protons through ILG, protonation remains a big challenge for many others. Furthermore, the mechanism of proton intercalation from the ionic liquid/solid interface to whole film has not yet been revealed. Here, with a model system of inverse spinel NiCo O , an increase in system temperature during ILG forms a single but effective method to efficiently achieve protonation. Moreover, the ILG induces a novel phase transformation in NiCo O from ferrimagnetic metallic into antiferromagnetic insulating with protonation at elevated temperatures. This study shows that environmental temperature is an efficient tuning knob to manipulate ILG-induced ionic evolution.
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JCR | SNIP | JCR | SNIP | JCR | SNIP | JCR | SNIP |
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in: SICRIS
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