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Matsuno, J; Ihara, K; Yamamura, S; Wadati, H; Ishii, K; Shankar, V V; Kee, Hae-Young; Takagi, H
Physical review letters, 2015-Jun-19, Letnik: 114, Številka: 24Journal Article
In 5d Ir oxides with an interplay of spin-orbit coupling and electron correlations, we have tailored a spin-orbital magnetic insulator out of a semimetal SrIrO(3) by tuning the structure through superlattices (SrIrO(3))(m), SrTiO(3) (m=1,2,3,4, and ∞). We observed the systematic decrease of the magnetic ordering temperature and the resistivity as a function of m. The transition from the semimetal to the insulator is found to be closely linked to the appearance of magnetism at m≃3. Long range magnetic ordering was realized even in the m=1 single layer superlattice, implying that the design and realization of novel electronic phases is feasible at the level of a single atomic layer in complex Ir oxides.
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