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Kim, Jongjin B.; Weichman, Marissa L.; Sjolander, Tobias F.; Neumark, Daniel M.; Kłos, Jacek; Alexander, Millard H.; Manolopoulos, David E.
Science (American Association for the Advancement of Science), 07/2015, Letnik: 349, Številka: 6247Journal Article
Photodetachment spectroscopy of the FH2– and FD2– anions allows for the direct observation of reactive resonances in the benchmark reaction F + H2 → HF + H. Using cooled anion precursors and a high-resolution electron spectrometer, we observe several narrow peaks not seen in previous experiments. Theoretical calculations, based on a highly accurate F + H2 potential energy surface, convincingly assign these peaks to resonances associated with quasibound states in the HF + H and DF + D product arrangements and with a quasibound state in the transition state region of the F + H2 reaction. The calculations also reveal quasibound states in the reactant arrangement, which have yet to be resolved experimentally.
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JCR | SNIP | JCR | SNIP | JCR | SNIP | JCR | SNIP |
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in: SICRIS
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