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Dai, Jie; Zhu, Yinlong; Chen, Yu; Wen, Xue; Long, Mingce; Wu, Xinhao; Hu, Zhiwei; Guan, Daqin; Wang, Xixi; Zhou, Chuan; Lin, Qian; Sun, Yifei; Weng, Shih-Chang; Wang, Huanting; Zhou, Wei; Shao, Zongping
Nature communications, 03/2022, Letnik: 13, Številka: 1Journal Article
Improving the catalytic efficiency of platinum for the hydrogen evolution reaction is valuable for water splitting technologies. Hydrogen spillover has emerged as a new strategy in designing binary-component Pt/support electrocatalysts. However, such binary catalysts often suffer from a long reaction pathway, undesirable interfacial barrier, and complicated synthetic processes. Here we report a single-phase complex oxide La Sr PtO as a high-performance hydrogen evolution electrocatalyst in acidic media utilizing an atomic-scale hydrogen spillover effect between multifunctional catalytic sites. With insights from comprehensive experiments and theoretical calculations, the overall hydrogen evolution pathway proceeds along three steps: fast proton adsorption on O site, facile hydrogen migration from O site to Pt site via thermoneutral La-Pt bridge site serving as the mediator, and favorable H desorption on Pt site. Benefiting from this catalytic process, the resulting La Sr PtO exhibits a low overpotential of 13 mV at 10 mA cm , a small Tafel slope of 22 mV dec , an enhanced intrinsic activity, and a greater durability than commercial Pt black catalyst.
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Dostop do baze podatkov JCR je dovoljen samo uporabnikom iz Slovenije. Vaš trenutni IP-naslov ni na seznamu dovoljenih za dostop, zato je potrebna avtentikacija z ustreznim računom AAI.
Leto | Faktor vpliva | Izdaja | Kategorija | Razvrstitev | ||||
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JCR | SNIP | JCR | SNIP | JCR | SNIP | JCR | SNIP |
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Vir: Osebne bibliografije
in: SICRIS
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