Knowledge regarding microseismic characteristics associated with longwall coal mining is crucial in evaluating the potential for underground mining hazards. Although microseismicity is induced by ...mining activities, it still remains uncertain as to what extent mining activities influence the spatial, temporal, and magnitude characteristics of microseismicity. To establish a thorough understanding of the relationship between microseismic characteristics and mining activities, a 27-month long microseismic monitoring campaign was conducted around a highly stressed coal zone and eight producing longwall panels at Coal Mine Velenje in Slovenia. Each microseismic event was classified to be associated with the producing longwall panel that triggered it, and the microseismic response to multi-panel longwall top coal caving face advance was analysed. Monitoring data have shown that locations of microseismic events coincided with stress concentrated regions. It was established that both seismic count and energy-intensive regions associated with coal mining in different panels are spatially connected, but they do not fully overlap with mined-out or stress concentrated areas. In addition, microseismic event counts frequency was found to be well correlated with mining intensity, while seismic energy magnitude and spatial distribution are poorly correlated with the same. Therefore, microseismic characteristics could not be explained solely by the mining-induced stress transfer and mining intensity, but are believed to be dominated by pre-existing natural fractures throughout the coal seam. Analyses of these observations helped the development of a conceptual seismic-generation model, which provides new insights into the causes of microseismicity in coal mining.
A multi-objective optimisation model for CCS chains, aiming to minimise costs and greenhouse gas emissions, considering various transport options is presented. The model builds upon previous work and ...covers the CCS chain elements after CO2 is captured, including conditioning, pipeline and batch-wise transportation, intermediate hub storage and injection at CO2 storage fields. A prospective Life Cycle Inventory is integrated to evaluate emissions from batch-wise transportation. The model is parameterised for accurate estimations based on site-specific characteristics and is implemented in two standalone CCS chains, that are analogues to the Northern Lights project with dominant ship transport and the Stella Maris concept with direct injection ship transport, also incorporating distinct emission profiles, intermediate storage hubs and injection sites. A third implementation combining both chain concepts is implemented. By increasing in a step-wise manner the weight of the emissions in the objective function, the model evaluates cost and emission trade-offs. The optimisation selects costlier wells to minimise emissions and shifts from batch-wise ships to cross-continent pipelines. Chain emissions decrease over time with CO2 supply increase. Shipping operation dominates emissions, followed by well construction and infrastructure construction. Across all the implementations, the GHG emission intensity of the chain, after CO2 is captured, ranged from 3.3 to 14.2 %, depending on the concept and transport option adopted and accounting for regional characteristics (i.e., the electricity supply mix per country).
Geological storage of CO2 in saline aquifers and depleted oil and gas reservoirs can help mitigate CO2 emissions. However, CO2 leakage over a long storage period represents a potential concern. ...Therefore, it is critical to establish a good understanding of the interactions between CO2–brine and cement–caprock/reservoir rock to ascertain the potential for CO2 leakage. Accordingly, in this work, we prepared a unique set of composite samples to resemble the cement–reservoir rock interface. A series of experiments simulating deep wellbore environments were performed to investigate changes in chemical, physical, mechanical, and petrophysical properties of the composite samples. Here, we present the characterisation of composite core samples, including porosity, permeability, and mechanical properties, determined before and after long-term exposure to CO2-rich brine. Some of the composite samples were further analysed by X-ray microcomputed tomography (X-ray µ-CT), X-ray diffraction (XRD), and scanning electron microscopy–energy-dispersive X-ray (SEM–EDX). Moreover, the variation of ions concentration in brine at different timescales was studied by performing inductively coupled plasma (ICP) analysis. Although no significant changes were observed in the porosity, permeability of the treated composite samples increased by an order of magnitude, due mainly to an increase in the permeability of the sandstone component of the composite samples, rather than the cement or the cement/sandstone interface. Mechanical properties, including Young’s modulus and Poisson’s ratio, were also reduced.
This paper reports a numerical simulation study of a full CO2 core flooding and imbibition cycle on a Berea sandstone core (measured 14.45 cm long and 3.67 cm in diameter). During the test, ...supercritical CO2 (at 10 MPa and 40 °C) and CO2-saturated brine was injected into one end of the horizontal core and a X-ray CT scanner (with a resolution of 0.35 mm × 0.35 mm) was employed to monitor and record changes in the fluid saturations, which enabled 3D mapping of the saturation profiles throughout the core during the course of core flooding test. From the digital CT saturation data, mean saturation profiles along the core length were plotted with time. A 1D model of the core was constructed to simulate the core flooding test and attempt was made to history match core test results, particularly the evolution of the mean CO2 saturation profiles during CO2 injection. Curve-fitting of the centrifugal air-water capillary pressure data (drainage) for the Berea core showed that the core test data could be adequately described by the Van Genuchten equation. The matched set of parameters (Slr, P0, m) were 0.09, 20 KPa, 0.425 respectively. In the absence of the relative permeability for the Berea core, it was decided to use the parameters obtained from matching the air-water capillary pressure data as a first approximation for the CO2-brine system in the model.
In this study distributed optic fiber has been used to measure both the Rayleigh and Brillouin frequency shift of two different sandstone core samples under controlled hydrostatic confining and pore ...pressure in the laboratory. The Berea sandstone core is relatively homogeneous, whereas the Tako sandstone core is visibly heterogeneous with a coarse-grain and a fine-grain region. Rayleigh frequency has been found to have a superior performance over Brillouin frequency in terms of better consistency (less scattering) in the tests carried out. The strain gauge readings reveal considerable anisotropy in the stiffness of the Berea core between perpendicular (vertical) and parallel to the bedding (hoop) directions. The strains converted from Rayleigh frequency shift measurements agree reasonably well with readings by one of the four hoop strain gauge channels under increasing confining/pore pressure. For the Tako sandstone core, the contrast in the grain-size, and thus rock elastic properties, is clearly reflected in the hoop strain measurement by both strain gauges and distributed optic fiber. The outcomes of the test have demonstrated successfully the use of a single optic fiber for measuring rock strain response at different regions of a heterogeneous core sample along a continuous trajectory.
As part of a seismic monitoring project in a geothermal field, where the feasibility of re-injection and storage of produced CO2 is being investigated, a P- and S-wave seismic velocity ...characterisation study was carried out. The effect of axial (up to 95 MPa) and radial (up to 60 MPa) stress on the seismic velocity was studied in the laboratory for a broad range of dry sedimentary and metamorphic rocks that make up the Kızıldere geothermal system in Turkey. Thin section texture analyses conducted on the main reservoir formations, i.e., marble and calcschist, confirm the importance of the presence of fractures in the reservoir: 2D permeability increases roughly by a factor 10 when fractures are present. Controlled acoustic-assisted unconfined and confined compressive strength experiments revealed the stress-dependence of seismic velocities related to the several rock formations. For each test performed, a sharp increase in velocity was observed at relatively low absolute stress levels, as a result of the closure of microcracks, yielding an increased mineral-to-mineral contact area, thus velocity. A change in radial stress appeared to have a negligible impact on the resulting P-wave velocity, as long as it exceeds atmospheric pressure. The bulk of the rock formations studied showed reducing P-wave velocities as function of increasing temperature due to thermal expansion of the constituting minerals. This effect was most profound for the marble and calcschist samples investigated.
The TOPS project takes a radical and holistic approach to coupled UCG-CCS, and thus the site selection criteria for the coupled processes, considering both geological, reservoir and process ...engineering aspects and different end-uses of the produced synthetic gas in order to optimise the whole value chain. In particular, the experimental research carried out utilises a newly constructed high pressure gasification reactor investigating several prospective options of UCG technology implementations. Integrated research addresses field based technology knowledge gaps, such as cavity progression and geomechanics, potential groundwater contamination and subsidence impacts, together with research into process engineering solutions in order to assess the role/impact of site specific factors and selected reagents on the operability of given CO2 emission mitigation options. Ultimately, research aims to minimise the need for on-site CO2 storage capacity as well as maximising the economic yield of UCG through value added end products.
The urgency of climate change, while the world economy is projected to depend on fossil fuels for some time, requires substantial reduction of greenhouse gas emissions in the oil and gas industry. ...This study proposes a methodology for the decarbonisation of offshore natural gas production networks through progressive electrification, either by connecting offshore platforms with nearby renewable energy sources, e.g. offshore wind farms, or by sharing resources so as to improve their energy generation efficiency. In this context, a novel multi-objective mixed-integer linear programming model is proposed to simultaneously minimise greenhouse gas emissions and associated costs from a determined offshore platform network, considering technical constraints, such as maintaining the energy balance of the network, ensuring that cables are installed to enable energy flows, and respecting the maximum generation capacities and minimum operating loads of turbines. For demonstration purposes, the proposed methodology was applied to a UK Southern North Sea network and optimised using the augmented ε-constraint method. The Pareto front approximation obtained suggests that the studied network’s cumulative greenhouse gas emissions can be reduced by 25% over the next 10 years at an average cost of US$370.9 per tonne CO2e. This study also explores the impact that uncertainties and postponing investment decisions may have in the set context.
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•Offshore natural gas production GHG emissions can be reduced via electrification.•Energy generation options were analysed using a multi-objective optimisation model.•Sharing power production reduces GHG emissions in mature offshore fields in the UK.•GHG emissions reduction (25%) is achieved at average cost of US$370.9/tonneCO2e.•Integration with offshore wind farms provided the greatest benefits in the optima.
•The lower energy content lignite produced a syngas with comparatively better energy efficiency.•Life cycle carbon footprint of UCG-IGCC plants depends more on the process driven syngas composition ...rather than the in-situ methane content.•Life cycle carbon footprint of conventional above ground coal fired power generation depends on the in-situ CH4 content and CH4 emissions during mining.•Bituminous coal UCG-IGCC plants have a greater life cycle carbon footprint than that of lignite UCG-IGCC plants.•UCG methanol production and CCS releases more life cycle CO2-eq emissions than UCG ammonia.
Underground coal gasification (UCG) has the potential to provide a source of energy or chemical feedstock derived from coal seams, where traditional mining methods are not suitable or are uneconomical. This paper presents the life cycle inventory models developed for the UCG processes and three alternative syngas utilisation options with and without CO2 capture and storage. The paper compares the life cycle carbon footprint of two different conventional above ground coal fired power generation options with UCG Integrated Gasification Combined Cycle power generation with/without CCS for two different lignites and one bituminous coal. One of the lignites is then used to compare the life cycle performance of different syngas utilisation options: power generation, ammonia production with power generation, and methanol production with power generation. It was found that the life cycle carbon footprint of conventional above ground coal fired power generation is very much dependent on the in-situ methane content of the coal used, and methane emissions experienced during mining and accompanying upstream processes, whereas the same for UCG-IGCC power depends more on the process dependent syngas composition. UCG methanol production with associated power and CCS is shown to release more life cycle CO2-eq emissions per tonne of lignite consumed than that of UCG ammonia production with associated power and CCS and UCG CCGT power generation with CCS. Furthermore, when chemicals production from UCG is considered as the main objective, the most substantial improvements in comparison to conventional methods are associated with UCG ammonia process per tonne of chemical produced.