Transport of air from the troposphere to the stratosphere occurs primarily in the tropics, associated with the ascending branch of the Brewer-Dobson circulation. Here, we identify the transport of ...air masses from the surface, through the Asian monsoon, and deep into the stratosphere, using satellite observations of hydrogen cyanide (HCN), a tropospheric pollutant produced in biomass burning. A key factor in this identification is that HCN has a strong sink from contact with the ocean; much of the air in the tropical upper troposphere is relatively depleted in HCN, and hence, broad tropical upwelling cannot be the main source for the stratosphere. The monsoon circulation provides an effective pathway for pollution from Asia, India, and Indonesia to enter the global stratosphere.
Unprecedented Arctic ozone loss in 2011 Manney, Gloria L; Santee, Michelle L; Rex, Markus ...
Nature (London),
10/2011, Volume:
478, Issue:
7370
Journal Article
Peer reviewed
Chemical ozone destruction occurs over both polar regions in local winter-spring. In the Antarctic, essentially complete removal of lower-stratospheric ozone currently results in an ozone hole every ...year, whereas in the Arctic, ozone loss is highly variable and has until now been much more limited. Here we demonstrate that chemical ozone destruction over the Arctic in early 2011 was--for the first time in the observational record--comparable to that in the Antarctic ozone hole. Unusually long-lasting cold conditions in the Arctic lower stratosphere led to persistent enhancement in ozone-destroying forms of chlorine and to unprecedented ozone loss, which exceeded 80 per cent over 18-20 kilometres altitude. Our results show that Arctic ozone holes are possible even with temperatures much milder than those in the Antarctic. We cannot at present predict when such severe Arctic ozone depletion may be matched or exceeded.
Abstract
To assess the performance of the most recent versions of the Global Precipitation Measurement (GPM) Integrated Multisatellite Retrievals for GPM (IMERG), namely, V05 and V06, in Arctic ...regions, comparisons with Environment and Climate Change Canada (ECCC) Climate Network stations north of 60°N were performed. This study focuses on the IMERG monthly final products. The mean bias and mean error-weighted bias were assessed in comparison with 25 precipitation gauge measurements at ECCC Climate Network stations. The results of this study indicate that IMERG generally detects higher precipitation rates in the Canadian Arctic than ground-based gauge instruments, with differences ranging up to 0.05 and 0.04 mm h
−1
for the mean bias and the mean error-weighted bias, respectively. Both IMERG versions perform similarly, except for a few stations, where V06 tends to agree slightly better with ground-based measurements. IMERG’s tendency to detect more precipitation is in good agreement with findings indicating that weighing gauge measurements suffer from wind undercatch and other impairing factors, leading to lower precipitation estimates. Biases between IMERG and ground-based stations were found to be slightly larger during summer and fall, which is likely related to the increased precipitation rates during these seasons. Correlations of both versions of IMERG with the ground-based measurements are considerably lower in winter and spring than during summer and fall, which might be linked to issues that passive microwave (PMW) sensors encounter over ice and snow. However, high correlation coefficients with medians of 0.75–0.8 during summer and fall are very encouraging for potential future applications.
The GEOS-Chem simulation of atmospheric CH4 was evaluated against observations from the Thermal and Near Infrared Sensor for Carbon Observations Fourier Transform Spectrometer (TANSO-FTS) on the ...Greenhouse Gases Observing Satellite (GOSAT), the Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS), and the Total Carbon Column Observing Network (TCCON). We focused on the model simulations at the 4∘×5∘ and 2∘×2.5∘ horizontal resolutions for the period of February–May 2010. Compared to the GOSAT, TCCON, and ACE-FTS data, we found that the 2∘×2.5∘ model produced a better simulation of CH4, with smaller biases and a higher correlation to the independent data. We found large resolution-dependent differences such as a latitude-dependent XCH4 bias, with higher column abundances of CH4 at high latitudes and lower abundances at low latitudes at the 4∘×5∘ resolution than at 2∘×2.5∘. We also found large differences in CH4 column abundances between the two resolutions over major source regions such as China. These differences resulted in up to 30 % differences in inferred regional CH4 emission estimates from the two model resolutions. We performed several experiments using 222Rn, 7Be, and CH4 to determine the origins of the resolution-dependent errors. The results suggested that the major source of the latitude-dependent errors is excessive mixing in the upper troposphere and lower stratosphere, including mixing at the edge of the polar vortex, which is pronounced at the 4∘×5∘ resolution. At the coarser resolution, there is weakened vertical transport in the troposphere at midlatitudes to high latitudes due to the loss of sub-grid tracer eddy mass flux in the storm track regions. The vertical air mass fluxes are calculated in the model from the degraded coarse-resolution wind fields and the model does not conserve the air mass flux between model resolutions; as a result, the low resolution does not fully capture the vertical transport. This produces significant localized discrepancies, such as much greater CH4 abundances in the lower troposphere over China at 4∘×5∘ than at 2∘×2.5∘. Although we found that the CH4 simulation is significantly better at 2∘×2.5∘ than at 4∘×5∘, biases may still be present at 2∘×2.5∘ resolution. Their importance, particularly in regards to inverse modeling of CH4 emissions, should be evaluated in future studies using online transport in the native general circulation model as a benchmark simulation.
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