We present an open-source software package WannierTools, a tool for investigation of novel topological materials. This code works in the tight-binding framework, which can be generated by another ...software package Wannier90 (Mostofi et al., 2008). It can help to classify the topological phase of a given material by calculating the Wilson loop, and can get the surface state spectrum, which is detected by angle resolved photoemission (ARPES) and in scanning tunneling microscopy (STM) experiments. It also identifies positions of Weyl/Dirac points and nodal line structures, calculates the Berry phase around a closed momentum loop and Berry curvature in a part of the Brillouin zone (BZ).
Program title:WannierTools
Program Files doi:http://dx.doi.org/10.17632/ygsmh4hyh6.1
Licensing provisions: GNU General Public Licence 3.0
Programming language: Fortran 90
External routines/libraries used:•BLAS (http://www/netlib.org/blas)•LAPACK (http://www.netlib.org/lapack)
Nature of problem: Identifying topological classifications of crystalline systems including insulators, semimetals, metals, and studying the electronic properties of the related slab and ribbon systems.
Solution method: Tight-binding method is a good approximation for solid systems. Based on that, Wilson loop is used for topological phase classification. The iterative Green’s function is used for obtaining the surface state spectrum.
Humans can naturally and effectively find salient regions in complex scenes. Motivated by this observation, attention mechanisms were introduced into computer vision with the aim of imitating this ...aspect of the human visual system. Such an attention mechanism can be regarded as a dynamic weight adjustment process based on features of the input image. Attention mechanisms have achieved great success in many visual tasks, including image classification, object detection, semantic segmentation, video understanding, image generation, 3D vision, multimodal tasks, and self-supervised learning. In this survey, we provide a comprehensive review of various attention mechanisms in computer vision and categorize them according to approach, such as channel attention, spatial attention, temporal attention, and branch attention; a related repository
https://github.com/MenghaoGuo/Awesome-Vision-Attentions
is dedicated to collecting related work. We also suggest future directions for attention mechanism research.
Quantum networks play an extremely important role in quantum information science, with application to quantum communication, computation, metrology, and fundamental tests. One of the key challenges ...for implementing a quantum network is to distribute entangled flying qubits to spatially separated nodes, at which quantum interfaces or transducers map the entanglement onto stationary qubits. The stationary qubits at the separated nodes constitute quantum memories realized in matter while the flying qubits constitute quantum channels realized in photons. Dedicated efforts around the world for more than 20 years have resulted in both major theoretical and experimental progress toward entangling quantum nodes and ultimately building a global quantum network. Here, the development of quantum networks and the experimental progress over the past two decades leading to the current state of the art for generating entanglement of quantum nodes based on various physical systems such as single atoms, cold atomic ensembles, trapped ions, diamonds with nitrogen‐vacancy centers, and solid‐state host doped with rare‐earth ions are reviewed. Along the way, the merits are discussed and the potential of each of these systems toward realizing a quantum network is compared.
Quantum networks linking multiple remote quantum nodes consist of quantum memories served as stationary quantum nodes and flying photonic qubits served as quantum channels. This review summarizes and discusses the state of the art and future challenges for constructing quantum networks in various physical systems like single neutral atoms, cold atomic ensembles, trapped ions, NV centers, and rare‐earth‐ion doped solids.
A porous liquid containing empty cavities has been successfully fabricated by surface engineering of hollow structures with suitable corona and canopy species. By taking advantage of the liquid‐like ...polymeric matrices as a separation medium and the empty cavities as gas transport pathway, this unique porous liquid can function as a promising candidate for gas separation. Moreover, such a facile synthetic strategy can be further extended to the fabrication of other types of nanostructure‐based porous liquid, opening up new opportunities for preparation of porous liquids with attractive properties for specific tasks.
Perforated liquids: Functionalizing hollow silica spheres with suitable polymer species can produce a porous liquid containing empty silica cavities. Taking advantage of their liquid‐like polymeric matrixes as the separation medium and the empty cavities as the gas transport pathway they can function as a promising candidates for gas separation.
Video stabilization techniques are essential for most hand-held captured videos due to high-frequency shakes. Several 2D-, 2.5D-, and 3D-based stabilization techniques have been presented previously, ...but to the best of our knowledge, no solutions based on deep neural networks had been proposed to date. The main reason for this omission is shortage in training data as well as the challenge of modeling the problem using neural networks. In this paper, we present a video stabilization technique using a convolutional neural network. Previous works usually propose an off-line algorithm that smoothes a holistic camera path based on feature matching. Instead, we focus on low-latency, real-time camera path smoothing that does not explicitly represent the camera path and does not use future frames. Our neural network model, called StabNet, learns a set of mesh-grid transformations progressively for each input frame from the previous set of stabilized camera frames and creates stable corresponding latent camera paths implicitly. To train the network, we collect a dataset of synchronized steady and unsteady video pairs via a specially designed hand-held hardware. Experimental results show that our proposed online method performs comparatively to the traditional off-line video stabilization methods without using future frames while running about 10 times faster. More importantly, our proposed StabNet is able to handle low-quality videos, such as night-scene videos, watermarked videos, blurry videos, and noisy videos, where the existing methods fail in feature extraction or matching.
Redirected walking (RDW) allows users to explore virtual environments in limited physical spaces by imperceptibly steering them away from obstacles and space boundaries. However, even with those ...techniques, the risk of collision cannot always be avoided. For such situations, resetting techniques have been proposed to provide an immediate adjustment of the physical walking direction of a user. Existing resetting techniques are either applied in-place, where the user changes orientation but stays in the same position or out-of-place methods where the user is guided to move from the current position to a safe location all while freezing the movement in the virtual world. While out-of-place methods have the potential to provide more freedom to user movements after resetting, current out-of-place methods do not provide enough guidance for the users to move to optimal locations. In this work, we propose a novel out-of-place resetting strategy that guides users to optimal physical locations with the most potential for free movement and a smaller amount of resetting required for their further movements. For this purpose, we calculate a heat map of the walking area according to the average walking distance using a simulation of the currently used RDW algorithm. Based on this heat map, we identify the most suitable position for a one-step reset within a predefined searching range and use this one as the reset point. Our results show that our method increases the average moving distance within one cycle of resetting. Furthermore, our resetting method can be applied to any physical area with obstacles. That means that RDW methods that were not suitable for such environments (e.g., Steer to Center) combined with our resetting can also be extended to such complex walking areas. In addition, we present a user interface to provide a similar visual experience between these methods, using a two-arrows indicator to help users adjust their position and direction.
Cerebral cortex expansion is a hallmark of mammalian brain evolution; yet, how increased neurogenesis is coordinated with structural and functional development remains largely unclear. The T-box ...protein TBR2/EOMES is preferentially enriched in intermediate progenitors and supports cortical neurogenesis expansion. Here we show that TBR2 regulates fine-scale spatial and circuit organization of excitatory neurons in addition to enhancing neurogenesis in the mouse cortex. TBR2 removal leads to a significant reduction in neuronal, but not glial, output of individual radial glial progenitors as revealed by mosaic analysis with double markers. Moreover, in the absence of TBR2, clonally related excitatory neurons become more laterally dispersed and their preferential synapse development is impaired. Interestingly, TBR2 directly regulates the expression of Protocadherin 19 (PCDH19), and simultaneous PCDH19 expression rescues neurogenesis and neuronal organization defects caused by TBR2 removal. Together, these results suggest that TBR2 coordinates neurogenesis expansion and precise microcircuit assembly via PCDH19 in the mammalian cortex.
Trifluoromethyl trifluoromethanesulfonate has proved to be an excellent reservoir of difluorophosgene and a promising click ligation for amines in the preparation of urea derivatives, heterocycles, ...and carbamoyl fluorides under metal‐ and additive‐free conditions. The reactions are rapid, efficient, selective, and versatile, and can be performed in benign solvents, giving products in excellent yields with minimal efforts for purification. The characteristics of the reactions meet the requirements of a click reaction. The use of trifluoromethyl trifluoromethanesulfonate as a click reagent is advantageous over other “CO” sources (e.g., TsOCF3, PhCO2CF3, CsOCF3, AgOCF3, and triphosgene) because this reagent is readily accessible; easy to scale up; and highly reactive, even under metal‐ and additive‐free conditions. It is anticipated that CF3SO3CF3 will be increasingly as important as SO2F2 as a click agent in future drug design and development.
Back to basics: Trifluoromethyl trifluoromethanesulfonate is a promising click reagent for amines in the preparation of urea derivatives, heterocycles, and carbamoyl fluorides under metal‐ and additive‐free conditions (see scheme). The click reactions are rapid, efficient, and selective, and simply carried out in benign solvents to afford products with minimal efforts for purification.
Self-assembly has emerged as a powerful approach to generating complex supramolecular architectures. Despite there being many crystalline frameworks reported in the solid state, the construction of ...highly soluble periodic supramolecular networks in a three-dimensional space is still a challenge. Here we demonstrate that the encapsulation motif, which involves the dimerization of two aromatic units within cucurbit8uril, can be used to direct the co-assembly of a tetratopic molecular block and cucurbit8uril into a periodic three-dimensional supramolecular organic framework in water. The periodicity of the supramolecular organic framework is supported by solution-phase small-angle X-ray-scattering and diffraction experiments. Upon evaporating the solvent, the periodicity of the framework is maintained in porous microcrystals. As a supramolecular 'ion sponge', the framework can absorb different kinds of anionic guests, including drugs, in both water and microcrystals, and drugs absorbed in microcrystals can be released to water with selectivity.
A convenient method for deoxyfluorination of aromatic and aliphatic carboxylic acids with CF3SO2OCF3 in the presence of a suitable base at room temperature has been developed. The reaction allows a ...straightforward access to a variety of acyl fluorides and proves that CF3SO2OCF3 is an effective deoxyfluorination reagent for carboxylic acids. The method features simplicity, expeditiousness, high efficiency, ease of handling, good functional group tolerance, a wide range of substrates, excellent yields of products, compatibility of many amine initiators, use of environmentally friendly reagents, and effortless removal of byproducts. This reaction represents the first utilization of trifluoromethyl trifluoromethanesulfonate as a fluorination reagent.
Amine‐triggered deoxyfluorination of carboxylic acids with CF3SO2OCF3 is described. The reaction proceeds rapidly at room temperature under metal‐free conditions to form various acyl fluorides in up to 97 % yield. This protocol represents the first utilization of trifluoromethyl trifluoromethanesulfonate as a convenient and efficient fluorination reagent.
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