•820 g LMO crystal grown by the Czochralski method.•LMO elastic properties and stress anisotropies evaluated.•Concave tail shape generates more stresses than convex ones.
A new technology for the ...mass production of lithium molybdate (Li2MoO4) crystals needed for the realization of the cryogenic neutrinoless double-beta decay detectors is under development within the framework of the CLYMENE project. Crystals with 4 and 5 cm in diameter were grown in two different Czochralski configurations. The first configuration, based on inductive heating of a RF coil coupled with a platinum crucible, was used to grow crystals of 4 cm in diameter. Bolometric tests performed with two samples cut from a 230 g crystal have shown less performances of the large sample (158 g), which had a cleavage, as compared to the small non-cracked sample (13.5 g). Numerical modeling was applied to investigate the temperature field in the furnace, the melt convection and thermo-elastic stresses in the crystal. Numerical results reveal 30% higher thermal stress at the bottom part of the ingot in the case of a concave shape of the crystal tail (experimental case) as compared to the case of a convex shaped tail. This could explain why the fracture started at the bottom part of the 230 g crystal boule, and highlights the importance of the crystal shape in the last stage of growth process. The furnace configuration used to grow 5 cm-diameter crystals was numerically optimized in order to reduce the thermal stress in the crystals. The first kg-mass Li2MoO4 ingot grown in the optimized configuration exhibit regular shape and good structural quality.
A
bstract
Neutrinoless double-beta decay is a key process in particle physics. Its experimental investigation is the only viable method that can establish the Majorana nature of neutrinos, providing ...at the same time a sensitive inclusive test of lepton number violation. CROSS (Cryogenic Rare-event Observatory with Surface Sensitivity) aims at developing and testing a new bolometric technology to be applied to future large-scale experiments searching for neutrinoless double-beta decay of the promising nuclei
100
Mo and
130
Te. The limiting factor in large-scale bolometric searches for this rare process is the background induced by surface radioactive contamination, as shown by the results of the CUORE experiment. The basic concept of CROSS consists of rejecting this challenging background component by pulse-shape discrimination, assisted by a proper coating of the faces of the crystal containing the isotope of interest and serving as energy absorber of the bolometric detector. In this paper, we demonstrate that ultra-pure superconductive Al films deposited on the crystal surfaces act successfully as pulse-shape modifiers, both with fast and slow phonon sensors. Rejection factors higher than 99.9% of
α
surface radioactivity have been demonstrated in a series of prototypes based on crystals of Li
2
MoO
4
and TeO
2
. We have also shown that point-like energy depositions can be identified up to a distance of
∼
1 mm from the coated surface. The present program envisions an intermediate experiment to be installed underground in the Canfranc laboratory (Spain) in a CROSS-dedicated facility. This experiment, comprising
∼
3
×
10
25
nuclei of
100
Mo, will be a general test of the CROSS technology as well as a worldwide competitive search for neutrinoless double-beta decay, with sensitivity to the effective Majorana mass down to 70 meV in the most favorable conditions.
A new R&D on lithium molybdate scintillators has begun within a project CLYMENE (Czochralski growth of Li2MoO4 crYstals for the scintillating boloMeters used in the rare EveNts sEarches). One of the ...main goals of the CLYMENE is a realization of a Li2MoO4 crystal growth line to be complementary to the one recently developed by LUMINEU in view of a mass production capacity for CUPID, a next-generation tonne-scale bolometric experiment to search for neutrinoless double-beta decay. In the present paper we report the investigation of performance and radiopurity of 158-g and 13.5-g scintillating bolometers based on a first large-mass (230 g) Li2MoO4 crystal scintillator developed within the CLYMENE project. In particular, a good energy resolution (2–7 keV FWHM in the energy range of 0.2–5 MeV), one of the highest light yield (0.97 keV/MeV) amongst Li2MoO4 scintillating bolometers, an efficient alpha particles discrimination (10σ) and potentially low internal radioactive contamination (below 0.2–0.3 mBq/kg of U/Th, but 1.4 mBq/kg of 210Po) demonstrate prospects of the CLYMENE in the development of high quality and radiopure Li2MoO4 scintillators for CUPID.
In this work, we want to highlight the potential of lithium as a target for spin-dependent dark matter search in cryogenic experiments, with a special focus on the low-mass region of the parameter ...space. We operated a prototype detector module based on a Formula omitted target crystal in an above-ground laboratory. Despite the high background environment, the detector sets a competitive limit on spin-dependent interactions of dark matter particles with protons and neutrons for masses between Formula omitted and Formula omitted.
In this work we present how to fabricate large-area (15 cm2), ultra-low threshold germanium bolometric photo-detectors and how to operate them to detect few (optical) photons. These detectors work at ...temperatures as low as few tens of mK and exploit the Neganov-Trofimov-Luke (NTL) effect. They are operated as charge-to-heat transducers: the heat signal is linearly increased by simply changing a voltage bias applied to special metal electrodes, fabricated onto the germanium absorber, and read by a (NTD-Ge) thermal sensor. We fabricated a batch of five prototypes and ran them in different facilities with dilution refrigerators. We carefully studied how impinging spurious infrared radiation impacts the detector performances, by shining infrared photons via optical-fiber-guided LED signals, in a controlled manner, into the bolometers. We hence demonstrated how the radiation-tightness of the test environment tremendously enhances the detector performances, allowing to set electrode voltage bias up to 90 volts without any leakage current and signal-to-noise gain as large as a factor 12 (for visible photons). As consequence, for the first time we could operate large-area NTD-Ge-sensor-equipped NTL bolometric photo-detectors capable to reach sub 10-eV baseline noise (RMS). Such detectors open new frontiers for rare-event search experiments based on low light yield Ge-NTD equipped scintillating bolometers, such the CUPID neutrinoless double-beta decay experiment.
Neutrinoless double-beta (
0
ν
β
β
) decay is a hypothetical rare nuclear transition (
T
1
/
2
>
10
25
–
10
26
year). Its observation would provide an important insight into the nature of neutrinos ...(Dirac or Majorana particle) demonstrating that the lepton number is not conserved. This decay can be investigated with bolometers embedding the double-beta decay isotope (
76
Ge
,
82
Se
,
100
Mo
,
116
Cd
,
130
Te
...), which perform as low-temperature calorimeters (few tens of mK) detecting particle interactions via a small temperature rise read out by a dedicated thermometer. Cryogenic Rare-event Observatory with Surface Sensitivity (CROSS) aims at the development of bolometric detectors (based on
Li
2
MoO
4
and
TeO
2
crystals) capable of discriminating surface
α
and
β
interactions by exploiting superconducting properties of Al film deposited on the detector surface. We report in this paper the results of tests on prototypes performed at CSNSM (Orsay, France) that showed the capability of a-few-
μ
m
-thick superconducting Al film deposited on crystal surface to discriminate surface
α
from bulk events, thus providing the detector with the required pulse shape discrimination capability. The CROSS technology would further improve the background suppression and simplify the detector construction (no auxiliary light detector is needed to reject alpha surface events) with a view to future competitive double-beta decay searches.
The first observation of coherent elastic neutrino-nucleus scattering (CEνNS), reported by the COHERENT Collaboration in 2017, paved the way for a new generation of experiments using reactor ν̄e and ...aiming at precisely measuring this process. In this context, the BASKET (Bolometers At Sub-KeV Energy Thresholds) R&D project investigates the use of cryogenic detectors for a reactor CEνNS experiment. This article reports on the first test of a Mo-doped lithium tungstate scintillating bolometer (⊘18 × 7 mm, 8 g), performed in an aboveground laboratory at CSNSM, Orsay (France). The detector bolometric performance (energy and time response, particle identification capabilities) and radiopurity have been studied and confirm the promising potential of lithium tungstate-based bolometric detectors for the measurement of CEνNS at reactors.
For the first time, a cadmium tungstate crystal scintillator enriched in$^{116}$ Cd has been succesfully tested as a scintillating bolometer. The measurement was performed above ground at a ...temperature of 18 mK. The crystal mass was 34.5 g and the enrichment level $\sim $ 82 %. Despite a substantial pile-up effect due to above-ground operation, the detector demonstrated high energy resolution (2–7 keV FWHM in 0.2–2.6 MeV $\gamma $ energy range and 7.5 keV FWHM at the$^{116}$ Cd double-beta decay transition energy of 2813 keV), a powerful particle identification capability and a high level of internal radio-purity. These results prove that cadmium tungstate is a promising detector material for a next-generation neutrinoless double-beta decay bolometric experiment, like that proposed in the CUPID project (CUORE Upgrade with Particle IDentification).
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