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Silva Fernandes, Jéssica; de Sousa Fernandes, David Douglas; Pistonesi, Marcelo Fabián; Gonçalves Dias Diniz, Paulo Henrique
Food chemistry, 09/2023, Letnik: 421Journal Article
Display omitted •A chemometrics-assisted color histogram-based system used for tea quality analysis;•Fingerprint signatures from digital images used as analytical information;•Multivariate chemometric approaches used for qualitative and quantitative analysis;•Sri Lankan black and Argentinean black and green teas were authenticated;•Good results for the determination of moisture, total polyphenols, and caffeine. Tea (Camellia sinensis) fraud has been frequently identified and involves tampering with the labelling of inferior products or without geographical origin certification and even mixing them with superior quality teas to mask an adulteration. Consequently, economic losses and health damage to consumers are observed. Thus, a Chemometrics-assisted Color Histogram-based Analytical System (CACHAS) was employed a simple, cost-effective, reliable, and green analytical tool to screen the quality of teas. Data-Driven Soft Independent Modeling of Class Analogy was used to authenticate their geographical origin and category simultaneously, recognizing correctly all Argentinean and Sri Lankan black teas and Argentinean green teas. For the determination of moisture, total polyphenols, and caffeine, Partial Least Squares obtained satisfactory predictive abilities, with values of root mean squared error of prediction (RMSEP) of 0.50, 0.788, and 0.25 mg kg−1, rpred of 0.81, 0.902, and 0.81, and relative error of prediction (REP) of 6.38, 9.031, and 14.58%., respectively. CACHAS proved to be a good alternative tool for environmentally-friendly non-destructive chemical analysis.
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